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Orientation-Dependent Exciton–Plasmon Coupling in Embedded Organic/Metal Nanowire Heterostructures

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    Orientation-Dependent Exciton–Plasmon Coupling in Embedded Organic/Metal Nanowire Heterostructures
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    † †Key Laboratory of Photochemistry, Institute of Chemistry and §Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China
    ‡ State Key Laboratory of Electronic Thin-Film and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 610054, China
    ∥ University of Chinese Academy of Sciences, Beijing 100049, China
    *E-mail: [email protected]
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    ACS Nano

    Cite this: ACS Nano 2017, 11, 10, 10106–10112
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    https://doi.org/10.1021/acsnano.7b04584
    Published September 20, 2017
    Copyright © 2017 American Chemical Society
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    Abstract

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    The excitation of surface plasmons by optical emitters based on exciton–plasmon coupling is important for plasmonic devices with active optical properties. It has been theoretically demonstrated that the orientation of exciton dipole can significantly influence the coupling strength, yet systematic study of the coupling process in nanostructures is still hindered by the lack of proper material systems. In this work, we have experimentally investigated the orientation-dependent exciton–plasmon coupling in a rationally designed organic/metal nanowire heterostructure system. The heterostructures were prepared by inserting silver nanowires into crystalline organic waveguides during the self-assembly of dye molecules. Structures with different exciton orientations exhibited varying coupling efficiencies. The near-field exciton–plasmon coupling facilitates the design of nanophotonic devices based on the directional surface plasmon polariton propagations.

    Copyright © 2017 American Chemical Society

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    The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acsnano.7b04584.

    • Structure and morphology (SEM images); fluorescence properties (spectrum, lifetime); experimental setup for the optical characterization are given in Figures S1–S12 (PDF)

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    ACS Nano

    Cite this: ACS Nano 2017, 11, 10, 10106–10112
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acsnano.7b04584
    Published September 20, 2017
    Copyright © 2017 American Chemical Society
    Request reuse permissions

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