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Direct Assembly of Large Area Nanoparticle Arrays
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    Direct Assembly of Large Area Nanoparticle Arrays
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    • Heyou Zhang
      Heyou Zhang
      ARC Centre of Excellence in Exciton Science, School of Chemistry, University of Melbourne, Parkville, Victoria 3010, Australia
      More by Heyou Zhang
    • Jasper Cadusch
      Jasper Cadusch
      School of Physics, University of Melbourne, Parkville, Victoria 3010, Australia
    • Calum Kinnear
      Calum Kinnear
      ARC Centre of Excellence in Exciton Science, School of Chemistry, University of Melbourne, Parkville, Victoria 3010, Australia
    • Timothy James
      Timothy James
      School of Physics, University of Melbourne, Parkville, Victoria 3010, Australia
      Reserve Bank of Australia, Craigieburn, Victoria 3064, Australia
    • Ann Roberts
      Ann Roberts
      School of Physics, University of Melbourne, Parkville, Victoria 3010, Australia
      More by Ann Roberts
    • Paul Mulvaney*
      Paul Mulvaney
      ARC Centre of Excellence in Exciton Science, School of Chemistry, University of Melbourne, Parkville, Victoria 3010, Australia
      *E-mail: [email protected]
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    ACS Nano

    Cite this: ACS Nano 2018, 12, 8, 7529–7537
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    https://doi.org/10.1021/acsnano.8b02932
    Published July 13, 2018
    Copyright © 2018 American Chemical Society

    Abstract

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    A major goal of nanotechnology is the assembly of nanoscale building blocks into functional optical, electrical, or chemical devices. Many of these applications depend on an ability to optically or electrically address single nanoparticles. However, positioning large numbers of single nanocrystals with nanometer precision on a substrate for integration into solid-state devices remains a fundamental roadblock. Here, we report fast, scalable assembly of thousands of single nanoparticles using electrophoretic deposition. We demonstrate that gold nanospheres down to 30 nm in size and gold nanorods <100 nm in length can be assembled into predefined patterns on transparent conductive substrates within a few seconds. We find that rod orientation can be preserved during deposition. As proof of high fidelity scale-up, we have created centimeter scale patterns comprising more than 1 million gold nanorods.

    Copyright © 2018 American Chemical Society

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    The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acsnano.8b02932.

    • Additional information on single nanoparticle electrophoretic deposition cell assembly, gold nanoparticle scattering spectrum, structure characterization of single nanoparticle arrays (PDF)

    • Movie of the EPD deposition viewed in real time in a dark field microscope (MOV)

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    Cite this: ACS Nano 2018, 12, 8, 7529–7537
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    https://doi.org/10.1021/acsnano.8b02932
    Published July 13, 2018
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