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ACS Publications. Most Trusted. Most Cited. Most Read
An Ultrastretchable and Self-Healable Nanocomposite Conductor Enabled by Autonomously Percolative Electrical Pathways

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Download Hi-Res ImageDownload to MS-PowerPointCite This:ACS Nano 2019, 13, 6, 6531-6539
    Article

    An Ultrastretchable and Self-Healable Nanocomposite Conductor Enabled by Autonomously Percolative Electrical Pathways
    Click to copy article linkArticle link copied!

    • Sun Hong Kim
      Sun Hong Kim
      Department of Electrical and Computer Engineering, Inter-University Semiconductor Research Center, Seoul National University, 1-Gwanak-ro, Gwanak-gu, Seoul 08826, Republic of Korea
      More by Sun Hong Kim
    • Hyunseon Seo
      Hyunseon Seo
      Biomedical Research Institute, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea
      More by Hyunseon Seo
    • Jiheong Kang
      Jiheong Kang
      Department of Chemical Engineering, Stanford University, Stanford, California 94305-5025, United States
      More by Jiheong Kang
    • Jaeyoung Hong
      Jaeyoung Hong
      Advanced Analysis Center, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea
      More by Jaeyoung Hong
    • Duhwan Seong
      Duhwan Seong
      Biomedical Research Institute, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea
      More by Duhwan Seong
    • Han-Jin Kim
      Han-Jin Kim
      Department of Materials Science and Engineering, Korea University, Seoul 02841, Republic of Korea
      More by Han-Jin Kim
    • Jaemin Kim
      Jaemin Kim
      Department of Chemical Engineering, Stanford University, Stanford, California 94305-5025, United States
      More by Jaemin Kim
    • Jaewan Mun
      Jaewan Mun
      Department of Chemical Engineering, Stanford University, Stanford, California 94305-5025, United States
      More by Jaewan Mun
    • Inchan Youn
      Inchan Youn
      Biomedical Research Institute, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea
      More by Inchan Youn
      Orcidhttp://orcid.org/0000-0002-0977-0808
    • Jinseok Kim
      Jinseok Kim
      Biomedical Research Institute, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea
      More by Jinseok Kim
    • Yu-Chan Kim
      Yu-Chan Kim
      Biomedical Research Institute, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea
      More by Yu-Chan Kim
    • Hyun-Kwang Seok
      Hyun-Kwang Seok
      Biomedical Research Institute, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea
      More by Hyun-Kwang Seok
    • Changhee Lee
      Changhee Lee
      Department of Electrical and Computer Engineering, Inter-University Semiconductor Research Center, Seoul National University, 1-Gwanak-ro, Gwanak-gu, Seoul 08826, Republic of Korea
      More by Changhee Lee
      Orcidhttp://orcid.org/0000-0003-2800-8250
    • Jeffrey B.-H. Tok
      Jeffrey B.-H. Tok
      Department of Chemical Engineering, Stanford University, Stanford, California 94305-5025, United States
      More by Jeffrey B.-H. Tok
    • Zhenan Bao*
      Zhenan Bao
      Department of Chemical Engineering, Stanford University, Stanford, California 94305-5025, United States
      *E-mail: [email protected]
      More by Zhenan Bao
      Orcidhttp://orcid.org/0000-0002-0972-1715
    • Donghee Son*
      Donghee Son
      Biomedical Research Institute, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea
      *E-mail: [email protected]
      More by Donghee Son
      Orcidhttp://orcid.org/0000-0002-3772-8009
    Other Access OptionsSupporting Information (5)

    ACS Nano

    Cite this: ACS Nano 2019, 13, 6, 6531–6539
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    https://doi.org/10.1021/acsnano.9b00160
    Published May 9, 2019
    Copyright © 2019 American Chemical Society
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    Abstract

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    Abstract Image

    Both self-healable conductors and stretchable conductors have been previously reported. However, it is still difficult to simultaneously achieve high stretchability, high conductivity, and self-healability. Here, we observed an intriguing phenomenon, termed “electrical self-boosting”, which enables reconstructing of electrically percolative pathways in an ultrastretchable and self-healable nanocomposite conductor (over 1700% strain). The autonomously reconstructed percolative pathways were directly verified by using microcomputed tomography and in situ scanning electron microscopy. The encapsulated nanocomposite conductor shows exceptional conductivity (average value: 2578 S cm–1; highest value: 3086 S cm–1) at 3500% tensile strain by virtue of efficient strain energy dissipation of the self-healing polymer and self-alignment and rearrangement of silver flakes surrounded by spontaneously formed silver nanoparticles and their self-assembly in the strained self-healing polymer matrix. In addition, the conductor maintains high conductivity and stretchability even after recovered from a complete cut. Besides, a design of double-layered conductor enabled by the self-bonding assembly allowed a conducting interface to be located on the neutral mechanical plane, showing extremely durable operations in a cyclic stretching test. Finally, we successfully demonstrated that electromyogram signals can be monitored by our self-healable interconnects. Such information was transmitted to a prosthetic robot to control various hand motions for robust interactive human-robot interfaces.

    Copyright © 2019 American Chemical Society

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    Supporting Information

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    The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acsnano.9b00160.

    • Supplementary data (Figures S1–S35) and discussion (Notes S1–S4) (PDF)

    • Movie S1: A video showing a flexible wireless EMG recording system using a self-healable conductor as an interconnection laminated on skin (AVI)

    • Movie S2: A video showing real-time EMG monitoring using the flexible wireless EMG recording system (AVI)

    • Movie S3: A video showing repetitive stretching and releasing of the interconnect after completely cut and self-healed (AVI)

    • Movie S4: A video showing demonstration of human-robot interface (grabbing, slightly and fully spreading, and pointing) using the self-healed interconnect (AVI)

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    Cited By

    Click to copy section linkSection link copied!

    This article is cited by 101 publications.

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