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Probing Transient Localized Electromagnetic Fields Using Low-Energy Point-Projection Electron Microscopy

Cite this: ACS Photonics 2021, 8, 9, 2573–2580
Publication Date (Web):August 11, 2021
https://doi.org/10.1021/acsphotonics.1c00775
Copyright © 2021 The Authors. Published by American Chemical Society

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    Abstract

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    Low kinetic energy electrons are of interest for probing nanoscale dynamic processes using ultrafast electron microscopy techniques. Their low velocities reduce radiation doses and enhance the interaction with confined electromagnetic fields and, thus, may enable ultrafast spectroscopy of single nanostructures. Recent improvements in the spatial and temporal resolution of ultrafast, low-energy electron microscopy have been achieved by combining nanotip photoemitters and point-projection imaging schemes. Here, we use such an ultrafast point-projection electron microscope (UPEM) to analyze the interaction of low-energy electrons with transient electric fields created by photoemission from a nanogap antenna. By analyzing their kinetic energy distribution, we separate angular deflection due to radial field components from electron energy gain and loss due to their axial acceleration. Our measurements open up a route toward the spatial and temporal characterization of vectorial near-fields by low-energy electron streaking spectroscopy.

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    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acsphotonics.1c00775.

    • Single-crystalline gold tapers; Pasmonic nanoresonator; Electron detection and data handling; Spatial resolution; Local kinetic energy distribution; Temporal resolution; Simulation (PDF)

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    Cited By

    This article is cited by 8 publications.

    1. Pengzuo Jiang, Wei Zheng, Xiaofang Li, Linfeng Zhang, Yu Liu, Yang Wang, Yaolong Li, Yunan Gao, Hong Yang, Yunquan Liu, Qihuang Gong, Chengyin Wu. Imaging and Controlling Ultrafast Electron Pulses Emitted from Plasmonic Nanostructures. Nano Letters 2023, 23 (16) , 7327-7333. https://doi.org/10.1021/acs.nanolett.3c01644
    2. Andreas Wöste, Germann Hergert, Thomas Quenzel, Martin Silies, Dong Wang, Petra Groß, Christoph Lienau. Ultrafast Coupling of Optical Near Fields to Low-Energy Electrons Probed in a Point-Projection Microscope. Nano Letters 2023, 23 (12) , 5528-5534. https://doi.org/10.1021/acs.nanolett.3c00738
    3. Michael Yannai, Raphael Dahan, Alexey Gorlach, Yuval Adiv, Kangpeng Wang, Ivan Madan, Simone Gargiulo, Francesco Barantani, Eduardo J. C. Dias, Giovanni Maria Vanacore, Nicholas Rivera, Fabrizio Carbone, F. Javier García de Abajo, Ido Kaminer. Ultrafast Electron Microscopy of Nanoscale Charge Dynamics in Semiconductors. ACS Nano 2023, 17 (4) , 3645-3656. https://doi.org/10.1021/acsnano.2c10481
    4. Ivan Madan, Eduardo J. C. Dias, Simone Gargiulo, Francesco Barantani, Michael Yannai, Gabriele Berruto, Thomas LaGrange, Luca Piazza, Tom T. A. Lummen, Raphael Dahan, Ido Kaminer, Giovanni Maria Vanacore, F. Javier García de Abajo, Fabrizio Carbone. Charge Dynamics Electron Microscopy: Nanoscale Imaging of Femtosecond Plasma Dynamics. ACS Nano 2023, 17 (4) , 3657-3665. https://doi.org/10.1021/acsnano.2c10482
    5. Ann-Kathrin Raab, Marcus Seidel, Chen Guo, Ivan Sytcevich, Gunnar Arisholm, Anne L’Huillier, Cord L. Arnold, Anne-Lise Viotti. Multi-gigawatt peak power post-compression in a bulk multi-pass cell at a high repetition rate. Optics Letters 2022, 47 (19) , 5084. https://doi.org/10.1364/OL.463960
    6. Ivan Sytcevich, Anne-Lise Viotti, Chen Guo, Jan Vogelsang, Fabian Langer, Anne L’Huillier, Cord L. Arnold. Few-cycle short-wave-infrared light source for strong-field experiments at 200 kHz repetition rate. Optics Express 2022, 30 (15) , 27858. https://doi.org/10.1364/OE.460915
    7. Andreas Wöste, Germann Hergert, Martin Silies, Dong Wang, Petra Groß, Christoph Lienau. Photon-Induced Near-Field Interaction in Ultrafast Low Energy Electron Microscopy. 2022, Tu3A.5. https://doi.org/10.1364/UP.2022.Tu3A.5
    8. Germann Hergert, Andreas Wöste, Petra Groß, Christoph Lienau. Strong inelastic scattering of slow electrons by optical near fields of small nanostructures. Journal of Physics B: Atomic, Molecular and Optical Physics 2021, 54 (17) , 174001. https://doi.org/10.1088/1361-6455/ac2471

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