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Novel Sodium Niobate-Based Lead-Free Ceramics as New Environment-Friendly Energy Storage Materials with High Energy Density, High Power Density, and Excellent Stability

  • Mingxing Zhou
    Mingxing Zhou
    Key Laboratory of Inorganic Functional Materials and Devices, Shanghai Institute of Ceramics, Chinese Academy of Sciences, 588 Heshuo Road, Jiading District, Shanghai 201800, People’s Republic of China
    University of Chinese Academy of Sciences, 19 Yuquan Road, Shijinshan District, Beijing 100049, People’s Republic of China
    More by Mingxing Zhou
    Orcidhttp://orcid.org/0000-0002-1531-8201
    • , 
  • Ruihong Liang*
    Ruihong Liang
    Key Laboratory of Inorganic Functional Materials and Devices, Shanghai Institute of Ceramics, Chinese Academy of Sciences, 588 Heshuo Road, Jiading District, Shanghai 201800, People’s Republic of China
    *E-mail: [email protected]
    More by Ruihong Liang
    • , 
  • Zhiyong Zhou
    Zhiyong Zhou
    Key Laboratory of Inorganic Functional Materials and Devices, Shanghai Institute of Ceramics, Chinese Academy of Sciences, 588 Heshuo Road, Jiading District, Shanghai 201800, People’s Republic of China
    More by Zhiyong Zhou
    • , 
  • Shiguang Yan
    Shiguang Yan
    Key Laboratory of Inorganic Functional Materials and Devices, Shanghai Institute of Ceramics, Chinese Academy of Sciences, 588 Heshuo Road, Jiading District, Shanghai 201800, People’s Republic of China
    More by Shiguang Yan
    • , and 
  • Xianlin Dong*
    Xianlin Dong
    Key Laboratory of Inorganic Functional Materials and Devices, Shanghai Institute of Ceramics, Chinese Academy of Sciences, 588 Heshuo Road, Jiading District, Shanghai 201800, People’s Republic of China
    State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, 1295 Dingxi Road, Changning District, Shanghai 200050, People’s Republic of China
    *E-mail: [email protected]
    More by Xianlin Dong
Cite this: ACS Sustainable Chem. Eng. 2018, 6, 10, 12755–12765
Publication Date (Web):September 7, 2018
https://doi.org/10.1021/acssuschemeng.8b01926
Copyright © 2018 American Chemical Society
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Abstract

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Recently, ceramic capacitors with fast charge–discharge performance and excellent energy storage characteristics have received considerable attention. Novel NaNbO3-based lead-free ceramics (0.80NaNbO3-0.20SrTiO3, abbreviated as 0.80NN-0.20ST), featuring ultrahigh energy storage density, ultrahigh power density, and ultrafast discharge performance, were designed and prepared in this study. These 0.80NN-0.20ST ceramics exhibited a high breakdown strength of 323 kV/cm, attributable to their small grain size and dense microstructure, a recoverable energy storage density of 3.02 J/cm3, and an energy storage efficiency of 80.7% at an applied electric field of 310 kV/cm. The excellent stability of energy storage properties in frequency (0.1–1000 Hz), temperature (20–120 °C), and fatigue resistance (cycle number: 105) were also observed in the 0.80NN-0.20ST ceramics. In contrast with other recently reported lead-free ceramic-based dielectric capacitors, the 0.80NN-0.20ST ceramics display a high energy storage efficiency combined with a high recoverable energy storage density, which indicates that they have wide application foreground and potential in the field of energy storage. These ceramics also show a considerable current density of 677 A/cm2, an ultrahigh power density of 23.7 MW/cm3, and a short release duration (∼225 ns). This study brings the NaNbO3-based ceramics into a new chapter of research and application of energy storage dielectric capacitors.

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  • Cross-sectional SEM image, schematic diagram of pulsed charge–discharge and period time T, and variation of discharge time (PDF)

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  17. Mingxing Zhou, Ruihong Liang, Zhiyong Zhou, Xianlin Dong. Developing a novel high performance NaNbO 3 -based lead-free dielectric capacitor for energy storage applications. Sustainable Energy & Fuels 2020, 4 (3) , 1225-1233. https://doi.org/10.1039/C9SE00836E
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