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Stimuli-Responsive Hydrogel Membranes Coupled with Biocatalytic Processes

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Department of Chemistry and Biomolecular Science and NanoBio Laboratory (NABLAB), Clarkson University, Potsdam, New York 13699-5810
* E-mail: [email protected] (E.K.), [email protected] (S.M.).
Cite this: ACS Appl. Mater. Interfaces 2009, 1, 3, 532–536
Publication Date (Web):February 12, 2009
Copyright © 2009 American Chemical Society

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    Abstract Image

    A nanostructured signal-responsive thin hydrogel membrane was coupled with enzyme-based systems to yield “smart” multisignal-responsive hybrid systems with built-in “logic”. The enzyme systems transduce biochemical input signals into structural changes of the membrane, thus resulting in the amplification of the biochemical signals and their transformation into the gated transport of molecules through the membrane. Coupling of the biocatalytic systems with a stimuli-responsive membrane is a promising approach for the development of materials that can regulate transport and release of chemicals/drugs by receiving and processing the biochemical information via biochemical reactions.

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