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    Fluorescence of Syndiotactic Polystyrene/Trimethylbenzene Clathrate and Intercalate Co-Crystals
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    Dipartimento di Chimica, Università degli Studi di Salerno, via Ponte Don Melillo, I-84084 Fisciano (SA), Italy, Dipartimento di Chimica “Paolo Corradini”, Università di Napoli “Federico II”, Complesso di Monte S.Angelo, Via Cintia, I-80126 Napoli, Italy, and Istituto per la Sintesi Organica e la Fotoreattività del Consiglio Nazionale delle Ricerche, c/o Dipartimento di Chimica dell’Università di Ferrara, Via Borsari, 46 - 44100 Ferrara, Italy
    †Università degli Studi di Salerno.
    ‡Università di Napoli “Federico II”.
    §Università di Ferrara.
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    Chemistry of Materials

    Cite this: Chem. Mater. 2007, 19, 24, 6041–6046
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    https://doi.org/10.1021/cm071483+
    Published October 25, 2007
    Copyright © 2007 American Chemical Society
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    Abstract

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    The self-assembling of fluorescent guest molecules, with the δ nanoporous host crystalline phase of syndiotactic polystyrene (s-PS) films, reduces chromophore diffusivity. Moreover, the chromophore fluorescence can be largely perturbed by formation of suitable polymer co-crystals. In particular, by excitation at the absorbance maximum (≈265 nm), s-PS/1,3,5-trimethylbenzene clathrate co-crystals present a broad fluorescence band nearly centered at 300 nm, while the corresponding intercalate co-crystals present a red-shifted fluorescence band with maxima at 330, 340, and 355 nm. This red shifted fluorescence is possibly due to absorption of the primary fluorescence by ground state complexes, formed in the intercalate co-crystal. The enhanced and red-shifted fluorescence could be relevant for optical and optoelectronic applications.

    Copyright © 2007 American Chemical Society

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    Chemistry of Materials

    Cite this: Chem. Mater. 2007, 19, 24, 6041–6046
    Click to copy citationCitation copied!
    https://doi.org/10.1021/cm071483+
    Published October 25, 2007
    Copyright © 2007 American Chemical Society
    Request reuse permissions

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