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On the Sources of Methane to the Los Angeles Atmosphere

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† Division of Engineering and Applied Science, California Institute of Technology, Pasadena, California 91125, United States
‡ Division of Geological and Planetary Sciences, California Institute of Technology, Pasadena, California 91125, United States
§ Keck Institute for Space Studies, California Institute of Technology, Pasadena, California 91125, United States
∥ School of Physical Sciences, University of California − Irvine, Irvine, California 92697, United States
⊥ Rosenstiel School of Marine and Atmospheric Science, University of Miami, Miami, Florida 33149, United States
# School of Engineering and Applied Sciences and Department of Earth and Planetary Sciences, Harvard University, Cambridge, Massachusetts 02318, United States
∇ NASA Langley Research Center, Hampton, Virginia 23681, United States
○ Environmental Energy Technologies Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States
*Phone: 626-395-2447. E-mail: [email protected]
Cite this: Environ. Sci. Technol. 2012, 46, 17, 9282–9289
Publication Date (Web):August 1, 2012
https://doi.org/10.1021/es301138y
Copyright © 2012 American Chemical Society
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    Abstract

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    We use historical and new atmospheric trace gas observations to refine the estimated source of methane (CH4) emitted into California’s South Coast Air Basin (the larger Los Angeles metropolitan region). Referenced to the California Air Resources Board (CARB) CO emissions inventory, total CH4 emissions are 0.44 ± 0.15 Tg each year. To investigate the possible contribution of fossil fuel emissions, we use ambient air observations of methane (CH4), ethane (C2H6), and carbon monoxide (CO), together with measured C2H6 to CH4 enhancement ratios in the Los Angeles natural gas supply. The observed atmospheric C2H6 to CH4 ratio during the ARCTAS (2008) and CalNex (2010) aircraft campaigns is similar to the ratio of these gases in the natural gas supplied to the basin during both these campaigns. Thus, at the upper limit (assuming that the only major source of atmospheric C2H6 is fugitive emissions from the natural gas infrastructure) these data are consistent with the attribution of most (0.39 ± 0.15 Tg yr–1) of the excess CH4 in the basin to uncombusted losses from the natural gas system (approximately 2.5–6% of natural gas delivered to basin customers). However, there are other sources of C2H6 in the region. In particular, emissions of C2H6 (and CH4) from natural gas seeps as well as those associated with petroleum production, both of which are poorly known, will reduce the inferred contribution of the natural gas infrastructure to the total CH4 emissions, potentially significantly. This study highlights both the value and challenges associated with the use of ethane as a tracer for fugitive emissions from the natural gas production and distribution system.

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