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Epoxide Pathways Improve Model Predictions of Isoprene Markers and Reveal Key Role of Acidity in Aerosol Formation

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Download Hi-Res ImageDownload to MS-PowerPointCite This:Environ. Sci. Technol. 2013, 47, 19, 11056-11064
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    Epoxide Pathways Improve Model Predictions of Isoprene Markers and Reveal Key Role of Acidity in Aerosol Formation
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    † National Exposure Research Laboratory, US Environmental Protection Agency, Research Triangle Park, North Carolina, 27711 United States
    Department of Environmental Sciences and Engineering, University of North Carolina at Chapel Hill, North Carolina, 27599 United States
    § Alion Science and Technology, Box 12313, Research Triangle Park, North Carolina, 27709 United States
    *E-mail: [email protected]
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    Environmental Science & Technology

    Cite this: Environ. Sci. Technol. 2013, 47, 19, 11056–11064
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    https://doi.org/10.1021/es402106h
    Published August 26, 2013
    Copyright © 2013 American Chemical Society
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    Abstract

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    Isoprene significantly contributes to organic aerosol in the southeastern United States where biogenic hydrocarbons mix with anthropogenic emissions. In this work, the Community Multiscale Air Quality model is updated to predict isoprene aerosol from epoxides produced under both high- and low-NOx conditions. The new aqueous aerosol pathways allow for explicit predictions of two key isoprene-derived species, 2-methyltetrols and 2-methylglyceric acid, that are more consistent with observations than estimates based on semivolatile partitioning. The new mechanism represents a significant source of organic carbon in the lower 2 km of the atmosphere and captures the abundance of 2-methyltetrols relative to organosulfates during the simulation period. For the parametrization considered here, a 25% reduction in SOx emissions effectively reduces isoprene aerosol, while a similar reduction in NOx leads to small increases in isoprene aerosol.

    Copyright © 2013 American Chemical Society

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    Cite this: Environ. Sci. Technol. 2013, 47, 19, 11056–11064
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