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Adsorption Equilibrium and Kinetics of Water Vapor on Different Adsorbents

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    Adsorption Equilibrium and Kinetics of Water Vapor on Different Adsorbents
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    Laboratory of Separation and Reaction Engineering (LSRE), Department of Chemical Engineering, Faculty of Engineering, University of Porto, Rua Dr. Roberto Frias, s/n, 4200-465 Porto, Portugal, and Laboratory of Energy and Environment (LEMA), Department of Chemical Engineering and Food Engineering, Federal University of Santa Catarina, Campus Universitário, 88040-900 Florianópolis, SC, Brazil
    * To whom correspondence should be addressed. Phone + 351 22 508 1671. Fax: + 351 22 508 1674. E-mail: [email protected]
    †University of Porto.
    ‡Federal University of Santa Catarina.
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    Industrial & Engineering Chemistry Research

    Cite this: Ind. Eng. Chem. Res. 2008, 47, 18, 7019–7026
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    https://doi.org/10.1021/ie701732x
    Published August 13, 2008
    Copyright © 2008 American Chemical Society
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    Abstract

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    Water vapor needs to be removed from many industrial streams using, for example, adsorption processes. Equilibrium and kinetic data are essential for the design of these adsorption processes. In this work, the adsorption equilibrium isotherms of water vapor were measured at 303 K by a gravimetric system on three commercial adsorbents, an activated carbon, an activated alumina, and a zeolite. The zeolite sample presented the highest capacity at low relative pressures, while at pressures near saturation the higher amount adsorbed was obtained on the alumina sample. The experimental points obtained for the activated carbon and the zeolite were fitted with the Virial isotherm while the n-layer BET equation was used in the fitting of the alumina data. The adsorption kinetics was evaluated through the analysis of breakthrough curves obtained at the same temperature for different feed humidity values. The fixed bed behavior was described using an isothermal model that includes axial dispersion and external (film model) and internal (homogeneous LDF model) mass transfer resistances. The homogeneous diffusivity values were determined by adjusting the model to the experimental data.

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    Cite this: Ind. Eng. Chem. Res. 2008, 47, 18, 7019–7026
    Click to copy citationCitation copied!
    https://doi.org/10.1021/ie701732x
    Published August 13, 2008
    Copyright © 2008 American Chemical Society
    Request reuse permissions

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