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Indium Tin Oxide Nanoparticles with Compositionally Tunable Surface Plasmon Resonance Frequencies in the Near-IR Region

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Graduate School of Pure and Applied Sciences, University of Tsukuba, 1-1-1 Tennodai, Tsukuba, Ibaraki 305-8571, Japan
[email protected]; [email protected]
Cite this: J. Am. Chem. Soc. 2009, 131, 49, 17736–17737
Publication Date (Web):November 18, 2009
https://doi.org/10.1021/ja9064415
Copyright © 2009 American Chemical Society
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Here we report the synthesis of conducting indium tin oxide (ITO) nanoparticles (NPs) and their surface plasmon resonance (SPR) properties. The SPR peaks of the ITO NPs can be easily tuned by changing the concentration of Sn doping from 3 to 30 mol %. The shortest SPR wavelength of 1618 nm in 10% Sn-doped ITO NPs may reflect the highest electron carrier density in the ITO NPs. The controllable SPR frequencies of metal oxides may offer a novel approach for noble-metal-free SPR applications. Unlike noble-metal nanostructures, ITO has no inter- and intraband transitions in the vis−near-IR region and represents a free-electron conduction, allowing us to systematically study the origin of optical effects arising from the SPRs of conduction electrons.

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XRD patterns of ITO NPs and UV−vis−NIR spectra and XRD patterns of ITO NP films. This material is available free of charge via the Internet at http://pubs.acs.org.

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