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Solubility of CO2 in Sulfonate Ionic Liquids at High Pressure

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Group for Green Chemistry and Technology, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100080, People's Republic of China, and Department of Chemistry, Wesleyan University, Middletown, Connecticut 06459-0180
Cite this: J. Chem. Eng. Data 2005, 50, 1, 230–233
Publication Date (Web):December 15, 2004
https://doi.org/10.1021/je0497193
Copyright © 2005 American Chemical Society
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    Abstract

    In this work, the solubility of CO2 in sulfonate ionic liquids (ILs), such as trihexyl (tetradecyl) phosphonium dodecylbenzenesulfonates ([P6,6,6,14][C12H25PhSO3]) and trihexyl (tetradecyl) phosphonium mesylate ([P6,6,6,14][MeSO3]), was determined at temperatures ranging from (305 to 325) K and pressures ranging from (4 to 9) MPa. It was found that the difference of the solubility of CO2 in two kinds of sulfonate ILs is not dramatic on the basis of molality. The solubility of CO2 in [P6,6,6,14][MeSO3] is higher than that in [P6,6,6,14][C12H25PhSO3]. The solubility data were correlated by means of the extended Henry's law, and the thermodynamic functions, such as the standard enthalpy, standard Gibbs free energy, and standard entropy, were obtained. The Henry's law constant for CO2 in all the investigated ionic liquids increases with increasing temperature.

    *

    In papers with more than one author, the asterisk indicates the name of the author to whom inquiries about the paper should be addressed.

    †

     Chinese Academy of Sciences.

    ‡

     Wesleyan University.

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