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Densities and Volumetric Properties of Ethylene Glycol + Dimethylsulfoxide Mixtures at Temperatures of (278.15 to 323.15) K and Pressures of (0.1 to 100) MPa

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Institute of Solution Chemistry of Russian Academy of Sciences, Ivanovo, Russia
* To whom correspondence may be addressed. E-mail: [email protected]
Cite this: J. Chem. Eng. Data 2010, 55, 9, 3481–3488
Publication Date (Web):August 19, 2010
https://doi.org/10.1021/je100089s
Copyright © 2010 American Chemical Society

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    Abstract

    Densities, ρ, and compressibility coefficients, k = (vov)/vo, of ethylene glycol (1) + dimethylsulfoxide (2) mixtures were measured over the whole concentration range at pressures of (0.1 to 100) MPa and temperatures of (278.15 to 323.15) K. Excess molar volumes, isothermal compressibility, and thermal isobaric expansivity coefficients as well as thermal pressure coefficients were calculated. It was revealed that concentration dependences of specific volumes, v, at some state parameters passed a minimum. The shift of minimum position to molar fraction x2 = 0.5 was observed with increasing pressure and decreasing temperature. The negative excess molar volumes, VmE, indicated a compression of EG (1) + DMSO (2) systems when mixing. Composition dependences of isothermal compressibility, κT, and thermal isobaric expansivity coefficients, α, as well as thermal pressure coefficients, β, were near-linear. Both increasing and decreasing of κT and β values were observed with x2 increase depending on temperature and pressure magnitudes within the range of state parameters investigated.

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    The calculated coefficients of isothermal compressibility and coefficients of thermal isobaric expansivities of the ethylene glycol (1) + dimethylsulfoxide (2) mixture at temperatures of (278.15 to 323.15) K and pressures of (0.1 to 100) MPa are given Tables S1 and S2, respectively. This material is available free of charge via the Internet at http://pubs.acs.org.

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