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Phase Equilibrium of Binary Mixtures of n-Hexane + Branched Chlorobutanes: Experimental Results and Group Contribution Predictions
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    Phase Equilibrium of Binary Mixtures of n-Hexane + Branched Chlorobutanes: Experimental Results and Group Contribution Predictions
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    Departamento de Química Física, Facultad de Ciencias, Universidad de Zaragoza, 50009 Zaragoza, Spain
    Facultad de Ciencias de la Salud, Universidad San Jorge, Villanueva de Gállego, 50830, Zaragoza, Spain
    *Tel: +34976762295. Fax: +34976761202. E-mail: [email protected]
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    Journal of Chemical & Engineering Data

    Cite this: J. Chem. Eng. Data 2014, 59, 10, 3017–3024
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    https://doi.org/10.1021/je500116z
    Published June 2, 2014
    Copyright © 2014 American Chemical Society

    Abstract

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    In this work the study of the phase equilibrium (experimental and modeled) of three binary mixtures formed by n-hexane and a branched chlorobutane (2-chlorobutane, 1-chloro-2-methylpropane, or 2-chloro-2-methylpropane) is presented. New and consistent experimental vapor–liquid equilibrium data at isothermal conditions T = (288.15, 298.15, and 308.15) K have been obtained and correlated using the Wilson equation. In addition, two group contribution models, modified-UNIFAC (universal functional activity coefficient) and VTPR (volume-translated Peng–Robinson), have been used to predict the vapor–liquid equilibrium of the mixtures. The agreement between experimental results and predicted ones is not satisfactory.

    Copyright © 2014 American Chemical Society

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    Cited By

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    This article is cited by 4 publications.

    1. Najla Ben Mahdoui, Héctor Artigas, Carlos Lafuente, Monia Hichri, and Ismail Khattech . Isobaric Vapor–Liquid Equilibrium for the Binary Systems Dimethyl Disulfide + C1–C4 n-Alkanol at 40.000 and 101.325 kPa. Journal of Chemical & Engineering Data 2017, 62 (7) , 2037-2043. https://doi.org/10.1021/acs.jced.7b00078
    2. Najla Ben Mahdoui, Manuela Artal, Monia Hichri, Carlos Lafuente. Volumetric Behavior and Vapor–Liquid Equilibrium of Dimethyl Disulfide + n-Alkanol Binary Mixtures. Journal of Solution Chemistry 2019, 48 (1) , 1-14. https://doi.org/10.1007/s10953-019-00841-x
    3. Victor Antón, Santiago Martín, Carlos Lafuente, Ignacio Gascón. Experimental and predicted vapour–liquid equilibrium of the binary mixtures n-heptane + chlorobutane isomers. Fluid Phase Equilibria 2016, 409 , 72-77. https://doi.org/10.1016/j.fluid.2015.09.031
    4. J. Benito, H. Guerrero, H. Artigas, M.C. López, C. Lafuente. Refractive indices and static permittivities of systems containing n-hexane or n-heptane and isomeric chlorobutanes. The Journal of Chemical Thermodynamics 2015, 86 , 162-167. https://doi.org/10.1016/j.jct.2015.03.001

    Journal of Chemical & Engineering Data

    Cite this: J. Chem. Eng. Data 2014, 59, 10, 3017–3024
    Click to copy citationCitation copied!
    https://doi.org/10.1021/je500116z
    Published June 2, 2014
    Copyright © 2014 American Chemical Society

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