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Assessing the Salting-Out Behavior of Nitrobenzene, 2-Nitrotoluene, and 3-Nitrotoluene from Solubility Values in Pure Water and Seawater at Temperatures between (277 and 314) K

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Chemistry Department, United States Naval Academy, 572M Holloway Road, Annapolis, Maryland 21402
* Corresponding author. Phone: (410) 293-6339. Fax: (410) 293-2218. E-mail: [email protected]
†E-mail: [email protected].
Cite this: J. Chem. Eng. Data 2009, 54, 4, 1231–1235
Publication Date (Web):March 3, 2009
https://doi.org/10.1021/je800624c
Copyright © This article not subject to U.S. Copyright. Published 2009 by the American Chemical Society

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    Abstract

    The salting-out behavior of nitrobenzene (NB), 2-nitrotoluene (2-NT), and 3-nitrotoluene (3-NT) was determined from solubility measurements in pure water and seawater with ionic strengths = (0.1662, 0.3352, 0.5071, and 0.6820) mol·L−1 at temperatures between (277 and 314) K. For all compounds tested, the solubility increased with increasing temperature. Solubility values in pure water compare well with previously reported values. As the ionic strength of the solution increased, the solubility of the organic compounds decreased. The average salting-out coefficients for NB, 2-NT, and 3-NT were (0.12, 0.14, and 0.14) L·mol−1, respectively, which are consistent with measurements for other nitroaromatic compounds. Over the temperature range examined, the salting-out coefficients did not vary significantly.

    Cited By

    This article is cited by 9 publications.

    1. Alauddin Ahmed and Stanley I. Sandler . Temperature-Dependent Physicochemical Properties and Solvation Thermodynamics of Nitrotoluenes from Solvation Free Energies. Journal of Chemical & Engineering Data 2015, 60 (1) , 16-27. https://doi.org/10.1021/je500413a
    2. Dianne J. Luning Prak and Daniel W. O'Sullivan . Assessing the Salting-Out Behavior of 2,4-Dinitrobenzaldehyde and 2,6-Dinitrobenzaldehyde from Solubility Values in Pure Water and Seawater at Temperatures between (280 and 313) K. Journal of Chemical & Engineering Data 2011, 56 (5) , 2630-2633. https://doi.org/10.1021/je200134q
    3. Daniel W. O’Sullivan Jeffrey R. Denzel Dianne J. Luning Prak . Photolysis of 2,4,6-Trinitrotoluene in Seawater: Effect of Salinity and Nitrate Concentration. 2011, 157-169. https://doi.org/10.1021/bk-2011-1069.ch008
    4. Yizhak Marcus. On the solubility of non-ionic organic solutes in seawater. Pure and Applied Chemistry 2015, 87 (5) , 503-508. https://doi.org/10.1515/pac-2014-0908
    5. Sufian Alnemrat, Joseph P. Hooper. Predicting Solubility of Military, Homemade, and Green Explosives in Pure and Saline Water using COSMO‐RS. Propellants, Explosives, Pyrotechnics 2014, 39 (1) , 79-89. https://doi.org/10.1002/prep.201300071
    6. Leonid Gorb, Frances C. Hill, Yana Kholod, Eugeniy N. Muratov, Victor E. Kuz’min, Jerzy Leszczynski. Progress in Predictions of Environmentally Important Physicochemical Properties of Energetic Materials: Applications of Quantum-Chemical Calculations. 2012, 335-359. https://doi.org/10.1007/978-94-007-0923-2_9
    7. Mengjuan Li, Koichi Aoki, Jingyuan Chen, Toyohiko Nishiumi. Voltammetric determination of concentrations of ferrocene-included nitrobenzene droplets in water. Journal of Electroanalytical Chemistry 2011, 655 (2) , 159-163. https://doi.org/10.1016/j.jelechem.2011.02.015
    8. Yana A. Kholod, Ganna Gryn’ova, Leonid Gorb, Frances C. Hill, Jerzy Leszczynski. Evaluation of the dependence of aqueous solubility of nitro compounds on temperature and salinity: A COSMO-RS simulation. Chemosphere 2011, 83 (3) , 287-294. https://doi.org/10.1016/j.chemosphere.2010.12.065
    9. Israel Arias-González, Joel Reza, Arturo Trejo. Temperature and sodium chloride effects on the solubility of anthracene in water. The Journal of Chemical Thermodynamics 2010, 42 (11) , 1386-1392. https://doi.org/10.1016/j.jct.2010.06.006

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