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Xanthine Degradation and Related Enzyme Activities in Leaves and Fruits of Two Coffea Species Differing in Caffeine Catabolism
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    Xanthine Degradation and Related Enzyme Activities in Leaves and Fruits of Two Coffea Species Differing in Caffeine Catabolism
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    Departamento de Fisiologia Vegetal, Instituto de Biologia, Universidade Estadual de Campinas, CP6109, 13083-970 Campinas, SP, Brazil
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    Journal of Agricultural and Food Chemistry

    Cite this: J. Agric. Food Chem. 1999, 47, 5, 1851–1855
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    https://doi.org/10.1021/jf980892a
    Published April 30, 1999
    Copyright © 1999 American Chemical Society

    Abstract

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    The degradation of xanthine was studied in young and aged leaves and in immature and mature fruits of Coffeaarabica and Coffeadewevrei, which differ with respect to caffeine catabolism. Radioisotope feeding experiments showed that leaves degraded xanthine more readily than fruits but that mature fruits and aged leaves were less efficient than younger tissues. In all cases, a significant part of the recovered radioactivity was in the ureides. Xanthine dehydrogenase was characterized as the enzyme responsible for xanthine degradation, and its activity and that of uricase were consistent with the results obtained in the radioisotope feeding experiments. Activities of allantoinase and allantoate amidohydrolase could not be detected. Considerable levels of endogenous allantoin and allantoic acid were found in fruits and leaves. Therefore, ureide accumulation might be a consequence of low enzyme activity. There was no positive correlation between urease activity and the data from the radioisotope feeding experiments.

    Keywords: Allantoic acid; allantoin; Coffea arabica; Coffea dewevrei; uric acid; xanthine.

    Copyright © 1999 American Chemical Society

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    This article is cited by 13 publications.

    1. S. Irani, J. M. Lobo, G. R. Gray, C. D. Todd. Allantoin accumulation in response to increased growth irradiance in Arabidopsis thaliana. Biologia plantarum 2018, 62 (1) , 181-187. https://doi.org/10.1007/s10535-017-0747-2
    2. Estibaliz Urarte, Raquel Esteban, Jose Fernando Moran, Florian Bittner. Established and Proposed Roles of Xanthine Oxidoreductase in Oxidative and Reductive Pathways in Plants. 2015, 15-42. https://doi.org/10.1007/978-3-319-10079-1_2
    3. S. A. Fedoreyev, Y. V. Inyushkina, V. P. Bulgakov, M. V. Veselova, G. K. Tchernoded, A. V. Gerasimenko, Y. N. Zhuravlev. Production of allantoin, rabdosiin and rosmarinic acid in callus cultures of the seacoastal plant Mertensia maritima (Boraginaceae). Plant Cell, Tissue and Organ Culture (PCTOC) 2012, 110 (1) , 183-188. https://doi.org/10.1007/s11240-012-0125-x
    4. Thierry Joët, Eleanore T. Wurtzel, Fumio Matsuda, Kazuki Saito, Stéphane Dussert. Coupled Transcript-Metabolite Profiling: Towards Systems Biology Approaches to Unravel Regulation of Seed Secondary Metabolism. 2012, 367-385. https://doi.org/10.1007/978-94-007-4749-4_18
    5. Andre Rodrigues dos Reis, Jose Laercio Favarin, Luiz Antonio Gallo, Milton Ferreira Moraes, Tiago Tezotto, Jose Lavres Junior. INFLUENCE OF NITROGEN FERTILIZATION ON NICKEL ACCUMULATION AND CHEMICAL COMPOSITION OF COFFEE PLANTS DURING FRUIT DEVELOPMENT. Journal of Plant Nutrition 2011, 34 (12) , 1853-1866. https://doi.org/10.1080/01904167.2011.600412
    6. Paulo Mazzafera, Thomas W. Baumann, Milton Massao Shimizu, Maria Bernadete Silvarolla. Decaf and the Steeplechase Towards Decaffito—the Coffee from Caffeine-Free Arabica Plants. Tropical Plant Biology 2009, 2 (2) , 63-76. https://doi.org/10.1007/s12042-009-9032-7
    7. Paulo Mazzafera, Kátia Viviane Gonçalves, Milton Massao Shimizu. Control of Allantoin Accumulation in Comfrey. Natural Product Communications 2008, 3 (9) , 1934578X0800300. https://doi.org/10.1177/1934578X0800300905
    8. Sílvia B. Filippi, Ricardo A. Azevedo, Ladaslav Sodek, Paulo Mazzafera. Allantoin has a limited role as nitrogen source in cultured coffee cells. Journal of Plant Physiology 2007, 164 (5) , 544-552. https://doi.org/10.1016/j.jplph.2006.03.005
    9. P. Sauer, I. Frébort. Molybdenum Cofactor-Containing Oxidoreductase Family in Plants. Biologia plantarum 2003, 46 (4) , 481-490. https://doi.org/10.1023/A:1024814007027
    10. Pavel Sauer, Jitka Frébortová, Marek Šebela, Petr Galuszka, Susanne Jacobsen, Pavel Peč, Ivo Frébort. Xanthine dehydrogenase of pea seedlings: a member of the plant molybdenum oxidoreductase family. Plant Physiology and Biochemistry 2002, 40 (5) , 393-400. https://doi.org/10.1016/S0981-9428(02)01393-1
    11. H. R. Vega-Carrillo, F. Y. Iskander, E. Manzanares-Acuña. Elemental content in ground and soluble/instant coffee. Journal of Radioanalytical and Nuclear Chemistry 2002, 252 (1) , 75-80. https://doi.org/10.1023/A:1015235704300
    12. M. R. Sondahl, T. W. Baumann. Agronomy II: Developmental and Cell Biology. 2001, 202-223. https://doi.org/10.1002/9780470690499.ch10
    13. PAULO MAZZAFERA. Mineral nutrition and caffeine content in coffee leaves. Bragantia 1999, 58 (2) , 387-391. https://doi.org/10.1590/S0006-87051999000200018

    Journal of Agricultural and Food Chemistry

    Cite this: J. Agric. Food Chem. 1999, 47, 5, 1851–1855
    Click to copy citationCitation copied!
    https://doi.org/10.1021/jf980892a
    Published April 30, 1999
    Copyright © 1999 American Chemical Society

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