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Two-Photon Absorption Cross Section Determination for Fluorene Derivatives:  Analysis of the Methodology and Elucidation of the Origin of the Absorption Processes

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    Two-Photon Absorption Cross Section Determination for Fluorene Derivatives:  Analysis of the Methodology and Elucidation of the Origin of the Absorption Processes
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    Department of Chemistry and CREOL, College of Optics and Photonics, University of Central Florida, P.O. Box 162366, Orlando, Florida 32816-2366, and Institute of Physics National Academy of Sciences, Prospect Nauki 46, Kiev, 03028, Ukraine
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    The Journal of Physical Chemistry B

    Cite this: J. Phys. Chem. B 2007, 111, 44, 12723–12729
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    https://doi.org/10.1021/jp074456f
    Published October 16, 2007
    Copyright © 2007 American Chemical Society
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    Abstract

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    A comprehensive analysis of the well-known open aperture Z-scan method, using a modified equation for the change in transmittance, is presented and accounts for discrepancies in two-photon absorption (2PA) cross sections between picosecond and femtosecond excitation. This new approach takes into account excited-state absorption and stimulated emission of the molecules studied. The two-photon absorption cross-section spectra of a series of six fluorene-based derivatives, determined using picosecond pulses, over a broad spectral range (500−900 nm), and this approach using a modified fitting procedure in the open aperture Z-scan is reported. We demonstrate that the fluorene derivatives exhibit two-photon absorption cross-section values between 700 and 5000 GM, when excited into the two-photon allowed electronic state. Excitation anisotropy spectra, measured to investigate the nature of the observed linear and nonlinear absorption bands, are presented and provide insight into the 2PA process.

    Copyright © 2007 American Chemical Society

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     To whom correspondence should be addressed. Phone:  407-823-1028. E-mail:  [email protected].

    †

     Department of Chemistry.

    ‡

     CREOL.

    §

     Institute of Physics National Academy of Sciences.

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    The Journal of Physical Chemistry B

    Cite this: J. Phys. Chem. B 2007, 111, 44, 12723–12729
    Click to copy citationCitation copied!
    https://doi.org/10.1021/jp074456f
    Published October 16, 2007
    Copyright © 2007 American Chemical Society
    Request reuse permissions

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