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Anomalous Hysteresis in Perovskite Solar Cells

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Download Hi-Res ImageDownload to MS-PowerPointCite This:J. Phys. Chem. Lett. 2014, 5, 9, 1511-1515
    Energy Conversion and Storage; Energy and Charge Transport

    Anomalous Hysteresis in Perovskite Solar Cells
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    Department of Physics, University of Oxford, Clarendon Laboratory, Parks Road, Oxford OX1 3PU, United Kingdom
    *E-mail: [email protected]
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    The Journal of Physical Chemistry Letters

    Cite this: J. Phys. Chem. Lett. 2014, 5, 9, 1511–1515
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    https://doi.org/10.1021/jz500113x
    Published March 24, 2014
    Copyright © 2014 American Chemical Society
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    Abstract

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    Perovskite solar cells have rapidly risen to the forefront of emerging photovoltaic technologies, exhibiting rapidly rising efficiencies. This is likely to continue to rise, but in the development of these solar cells there are unusual characteristics that have arisen, specifically an anomalous hysteresis in the current–voltage curves. We identify this phenomenon and show some examples of factors that make the hysteresis more or less extreme. We also demonstrate stabilized power output under working conditions and suggest that this is a useful parameter to present, alongside the current-voltage scan derived power conversion efficiency. We hypothesize three possible origins of the effect and discuss its implications on device efficiency and future research directions. Understanding and resolving the hysteresis is essential for further progress and is likely to lead to a further step improvement in performance.

    Copyright © 2014 American Chemical Society

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    Supporting Information

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    Device fabrication and solar cell characterization details. Current–voltage characteristics. Scan rate dependence of the current–voltage characteristics of a mesosuperstructured perovskite solar cell and perovskite-sensitized solar cell. Current–voltage characteristics of a perovskite-sensitized solar cell. Extracted current density from a planar perovskite cell over time, when the cell is held at different voltage conditions until stabilized. This material is available free of charge via the Internet at http://pubs.acs.org.

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    This article is cited by 2211 publications.

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    Cite this: J. Phys. Chem. Lett. 2014, 5, 9, 1511–1515
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