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Dynamic Adhesion Forces between Microparticles and Substrates in Water

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Institute of New Energy, China University of Petroleum (Beijing), Beijing 102249, P. R. China
Department of Materials Science and Engineering and §Department of Chemistry, University of North Texas, Denton, Texas 76203, United States
International Research Center for “Solar-Hydrogen” Renewable and Clean Energy, State key Laboratory of Multiphase Flow in Power Engineering, Xi’an Jiaotong University, Xi’an, Shaanxi 710049, P. R. China
Cite this: Langmuir 2014, 30, 37, 11103–11109
Publication Date (Web):August 27, 2014
https://doi.org/10.1021/la502735w
Copyright © 2014 American Chemical Society
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Abstract

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The interactions between micrometer-sized particles and substrates in aqueous environment are fundamental to numerous natural phenomena and industrial processes. Here we report a dynamically induced enhancement in adhesion interactions between microparticles and substrates immerged in water, air, and hexane. The dynamic adhesion force was measured by pulling microsized spheres off various substrate (hydrophilic/hydrophobic) surfaces at different retracting velocities. It was observed that when the pull-off velocity varies from 0.02 to 1500 μm/s, there is 100–200% increase in adhesion force in water while it has a 100% increase in nitrogen and hexane. The dynamic adhesion enhancement reduces with increasing effective contact angle defined by the average cosine of wetting angles of the substrates and the particles, and approaches the values measured in dry nitrogen and hexane as the effective contact angle is larger than 90o. A dynamic model was developed to predict the adhesion forces resulting from this dynamic effect, and the predictions correlate well with the experimental results. The stronger dynamic adhesion enhancement in water is mainly attributed to electrical double layers and the restructuring of water in the contact area between particles and substrates.

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