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Ultrafast Dynamics of Surface-Enhanced Raman Scattering Due to Au Nanostructures

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†Interdisciplinary Research Center and ‡Graduate School of Engineering, Yokohama National University, Yokohama, Kanagawa 240-8501, Japan
Fritz-Haber-Institut der Max-Planck-Gesellschaft, 14195 Berlin, Germany
Institute of Physics, University of Tsukuba, Tsukuba, Ibaraki 305-8577, Japan
⊥Sensor Materials Center and #Advanced Nano-Characterization Center, National Institute for Materials Science, Tsukuba, Ibaraki 305-0047, Japan
Department of Applied Physics, National Defense Academy, Yokosuka, Kanagawa 239-8686, Japan
E-mail: [email protected]; [email protected]
Cite this: Nano Lett. 2011, 11, 7, 2648–2654
Publication Date (Web):May 23, 2011
https://doi.org/10.1021/nl200667t
Copyright © 2011 American Chemical Society
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Abstract

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Ultrafast dynamics of surface-enhanced Raman scattering (SERS) was investigated at cleaved graphite surfaces bearing deposited gold (Au) nanostructures (∼10 nm in diameter) by using sensitive pump–probe reflectivity spectroscopy with ultrashort (7.5 fs) laser pulses. We observed enhancement of phonon amplitudes (C═C stretching modes) in the femtosecond time domain, considered to be due to the enhanced electromagnetic (EM) field around the Au nanostructures. Finite-difference time-domain (FDTD) calculations confirmed the EM enhancement. The enhancement causes drastic increase of coherent D-mode (40 THz) phonon amplitude and nanostructure-dependent changes in the amplitude and dephasing time of coherent G-mode (47 THz) phonons. This methodology should be suitable to study the basic mechanism of SERS and may also find application in nanofabrication.

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