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Plasmon Hybridization in Individual Gold Nanocrystal Dimers: Direct Observation of Bright and Dark Modes

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† Department of Physics
§ Institute of Nanoengineering and Microsystems, National Tsing-Hua University, Hsinchu 30013, Taiwan
‡ Department of Chemistry, Graduate School of Pure and Applied Sciences, University of Tsukuba, 1-1-1 Tennodai, Tsukuba, Ibaraki 305-8571, Japan
* Corresponding author, [email protected]
Cite this: Nano Lett. 2010, 10, 2, 632–637
Publication Date (Web):January 8, 2010
https://doi.org/10.1021/nl903693v
Copyright © 2010 American Chemical Society
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Abstract

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We apply a nanomanipulation technique to assemble pairs of monodispersed octahedral gold nanocrystals (side length, 150 nm) along their major axes with a varying tip-to-tip separation (25−125 nm). These pairs are immobilized onto indium tin oxide coated silica substrates and studied as plasmonic dimers by polarization-selective total internal reflection (TIR) microscopy and spectroscopy. We confirm that the plasmon coupling modes with the scattering polarization along the incident light direction result from the transverse-magnetic-polarized incident light, which induces two near-field-coupled dipole moments oriented normal to the air−substrate interface. In such cases, both in-phase (antibonding) and antiphase (bonding) plasmon coupling modes can be directly observed with the incident light wave vector perpendicular and parallel to the dimer axis, respectively. The observation of antiphase plasmon coupling modes (“dark” plasmons) is made possible by the unique polarization nature of the TIR-generated evanescent field. Furthermore, with decreasing nanocrystal separation, the plasmon coupling modes shift to shorter wavelengths for the incident light perpendicular to the dimer axis, whereas relatively large red shifts of the plasmonic coupling modes are found for the parallel incident light.

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Additional information on synthesis of Au octahedra and polarization-selective microscattering spectroscopy using total internal reflection geometry and a video showing the actual dimer manipulation process. This material is available free of charge via the Internet at http://pubs.acs.org.

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