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Magnetic−Plasmonic Core−Shell Nanoparticles

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Department of Chemistry
Department of Physics and Astronomy
§ Department of Electrical and Computer Engineering, Rice University, P.O. Box 1892, Houston, Texas 77251-1892
* Address correspondence to [email protected]
Cite this: ACS Nano 2009, 3, 6, 1379–1388
Publication Date (Web):May 14, 2009
https://doi.org/10.1021/nn900118a
Copyright © 2009 American Chemical Society

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    Abstract

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    Nanoparticles composed of magnetic cores with continuous Au shell layers simultaneously possess both magnetic and plasmonic properties. Faceted and tetracubic nanocrystals consisting of wüstite with magnetite-rich corners and edges retain magnetic properties when coated with a Au shell layer, with the composite nanostructures showing ferrimagnetic behavior. The plasmonic properties are profoundly influenced by the high dielectric constant of the mixed iron oxide nanocrystalline core. A comprehensive theoretical analysis that examines the geometric plasmon tunability over a range of core permittivities enables us to identify the dielectric properties of the mixed oxide magnetic core directly from the plasmonic behavior of the core−shell nanoparticle.

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    Additional information includes a comparison of the electric field enhancement distribution for nanoshells with three different core shapes, a Raman spectrum of the iron oxide nanoparticles, magnetization measurements as a function of temperature, a histogram of the particles used for SQUID measurements, and XPS spectra of the iron oxide nanoparticles. This material is available free of charge via the Internet at http://pubs.acs.org.

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