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Air Quality and Health Impact of Future Fossil Fuel Use for Electricity Generation and Transport in Africa

  • Eloise A. Marais*
    Eloise A. Marais
    School of Physics and Astronomy, University of Leicester, Leicester, LE1 7RH, United Kingdom
    *E-mail: [email protected]
  • Rachel F. Silvern
    Rachel F. Silvern
    Department of Earth and Planetary Sciences, Harvard University, Cambridge, Massachusetts 02138, United States
  • Alina Vodonos
    Alina Vodonos
    Harvard T.H. Chan School of Public Health, Harvard University, Boston, Massachusetts 02115, United States
  • Eleonore Dupin
    Eleonore Dupin
    Department of Chemical Engineering, INSA, Cedex, 76800, France
  • Alfred S. Bockarie
    Alfred S. Bockarie
    School of Geography, Earth and Environmental Sciences, University of Birmingham, Birmingham, B15 2SA, United Kingdom
  • Loretta J. Mickley
    Loretta J. Mickley
    John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts 02138, United States
  • , and 
  • Joel Schwartz
    Joel Schwartz
    Harvard T.H. Chan School of Public Health, Harvard University, Boston, Massachusetts 02115, United States
Cite this: Environ. Sci. Technol. 2019, 53, 22, 13524–13534
Publication Date (Web):October 24, 2019
https://doi.org/10.1021/acs.est.9b04958
Copyright © 2019 American Chemical Society
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Supporting Info (2)»

Abstract

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Africa has ambitious plans to address energy deficits and sustain economic growth with fossil fueled power plants. The continent is also experiencing faster population growth than anywhere else in the world that will lead to proliferation of vehicles. Here, we estimate air pollutant emissions in Africa from future (2030) electricity generation and transport. We find that annual emissions of two precursors of fine particles (PM2.5) hazardous to health, sulfur dioxide (SO2) and nitrogen oxides (NOx), approximately double by 2030 relative to 2012, increasing from 2.5 to 5.5 Tg SO2 and 1.5 to 2.8 Tg NOx. We embed these emissions in the GEOS-Chem model nested over the African continent to simulate ambient concentrations of PM2.5 and determine the burden of disease (excess deaths) attributable to exposure to future fossil fuel use. We calculate 48000 avoidable deaths in 2030 (95% confidence interval: 6000–88000), mostly in South Africa (10400), Nigeria (7500), and Malawi (2400), with 3-times higher mortality rates from power plants than transport. Sensitivity of the burden of disease to either population growth or air quality varies regionally and suggests that emission mitigation strategies would be most effective in Southern Africa, whereas population growth is the main driver everywhere else.

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The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acs.est.9b04958.

  • Description of the attributable health calculation; the shape of the concentration–response function, evaluation of GEOS-Chem PM2.5; satellite observations of NO2 and SO2 over South Africa; and maps of GEOS-Chem surface ozone in 2012 and the change in 2030 relative to 2012 (PDF)

  • Location, generating capacity, air pollutant emissions, and data sources of power plants operating in 2012; operating, commissioned, undergoing construction, or proposed after 2012; air pollution, mortality, and sensitivity metrics for the 10 countries with highest mortality (XLSX)

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Most electronic Supporting Information files are available without a subscription to ACS Web Editions. Such files may be downloaded by article for research use (if there is a public use license linked to the relevant article, that license may permit other uses). Permission may be obtained from ACS for other uses through requests via the RightsLink permission system: http://pubs.acs.org/page/copyright/permissions.html.

Cited By


This article is cited by 15 publications.

  1. Alfred S. Bockarie, Eloise A. Marais, A. R. MacKenzie. Air Pollution and Climate Forcing of the Charcoal Industry in Africa. Environmental Science & Technology 2020, 54 (21) , 13429-13438. https://doi.org/10.1021/acs.est.0c03754
  2. , Euan G. Nisbet, Grant Allen, Rebecca E. Fisher, James L. France, James D. Lee, David Lowry, Marcos F. Andrade, Thomas J. Bannan, Patrick Barker, Prudence Bateson, Stéphane J.-B. Bauguitte, Keith N. Bower, Tim J. Broderick, Francis Chibesakunda, Michelle Cain, Alice E. Cozens, Michael C. Daly, Anita L. Ganesan, Anna E. Jones, Musa Lambakasa, Mark F. Lunt, Archit Mehra, Isabel Moreno, Dominika Pasternak, Paul I. Palmer, Carl J. Percival, Joseph R. Pitt, Amber J. Riddle, Matthew Rigby, Jacob T. Shaw, Angharad C. Stell, Adam R. Vaughan, Nicola J. Warwick, Shona E. Wilde. Isotopic signatures of methane emissions from tropical fires, agriculture and wetlands: the MOYA and ZWAMPS flights. Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences 2022, 380 (2215) https://doi.org/10.1098/rsta.2021.0112
  3. Jiayuan Wang, Abosede Sarah Alli, Sierra Clark, Allison Hughes, Majid Ezzati, Andrew Beddows, Jose Vallarino, James Nimo, Josephine Bedford-Moses, Solomon Baah, George Owusu, Ernest Agyemang, Frank Kelly, Benjamin Barratt, Sean Beevers, Samuel Agyei-Mensah, Jill Baumgartner, Michael Brauer, Raphael E. Arku. Nitrogen oxides (NO and NO2) pollution in the Accra metropolis: Spatiotemporal patterns and the role of meteorology. Science of The Total Environment 2022, 803 , 149931. https://doi.org/10.1016/j.scitotenv.2021.149931
  4. Sayyed Ahmad Khadem, Farid Bensebaa, Nathan Pelletier. Optimized feed-forward neural networks to address CO2-equivalent emissions data gaps – Application to emissions prediction for unit processes of fuel life cycle inventories for Canadian provinces. Journal of Cleaner Production 2022, 332 , 130053. https://doi.org/10.1016/j.jclepro.2021.130053
  5. Erin E. McDuffie, Randall V. Martin, Joseph V. Spadaro, Richard Burnett, Steven J. Smith, Patrick O’Rourke, Melanie S. Hammer, Aaron van Donkelaar, Liam Bindle, Viral Shah, Lyatt Jaeglé, Gan Luo, Fangqun Yu, Jamiu A. Adeniran, Jintai Lin, Michael Brauer. Source sector and fuel contributions to ambient PM2.5 and attributable mortality across multiple spatial scales. Nature Communications 2021, 12 (1) https://doi.org/10.1038/s41467-021-23853-y
  6. Danlu Zhang, Linlin Du, Wenhao Wang, Qingyang Zhu, Jianzhao Bi, Noah Scovronick, Mogesh Naidoo, Rebecca M. Garland, Yang Liu. A machine learning model to estimate ambient PM2.5 concentrations in industrialized highveld region of South Africa. Remote Sensing of Environment 2021, 266 , 112713. https://doi.org/10.1016/j.rse.2021.112713
  7. N.L. Rose, S.D. Turner, L.E. Unger, C.J. Curtis. The chronostratigraphy of the Anthropocene in southern Africa: Current status and potential. South African Journal of Geology 2021, 124 (4) , 1093-1106. https://doi.org/10.25131/sajg.124.0053
  8. F. Dettner, M. Blohm. External cost of air pollution from energy generation in Morocco. Renewable and Sustainable Energy Transition 2021, 24 , 100002. https://doi.org/10.1016/j.rset.2021.100002
  9. Caradee Y. Wright, Thandi Kapwata, David Jean du Preez, Bianca Wernecke, Rebecca M. Garland, Vusumuzi Nkosi, Willem A. Landman, Liesl Dyson, Mary Norval. Major climate change-induced risks to human health in South Africa. Environmental Research 2021, 196 , 110973. https://doi.org/10.1016/j.envres.2021.110973
  10. Alina Vodonos, Joel Schwartz. Estimation of excess mortality due to long-term exposure to PM2.5 in continental United States using a high-spatiotemporal resolution model. Environmental Research 2021, 196 , 110904. https://doi.org/10.1016/j.envres.2021.110904
  11. Karn Vohra, Alina Vodonos, Joel Schwartz, Eloise A. Marais, Melissa P. Sulprizio, Loretta J. Mickley. Global mortality from outdoor fine particle pollution generated by fossil fuel combustion: Results from GEOS-Chem. Environmental Research 2021, 195 , 110754. https://doi.org/10.1016/j.envres.2021.110754
  12. Philip Kofi Adom, Samuel Adams. Technical fossil fuel energy efficiency (TFFEE) and debt-finance government expenditure nexus in Africa. Journal of Cleaner Production 2020, 271 , 122670. https://doi.org/10.1016/j.jclepro.2020.122670
  13. Neil L. Rose, Alice M. Milner, Jennifer M. Fitchett, Kristy E. Langerman, Handong Yang, Simon D. Turner, Anne-Lise Jourdan, James Shilland, César C. Martins, Amanda Câmara de Souza, Christopher J. Curtis. Natural archives of long-range transported contamination at the remote lake Letšeng-la Letsie, Maloti Mountains, Lesotho. Science of The Total Environment 2020, 737 , 139642. https://doi.org/10.1016/j.scitotenv.2020.139642
  14. William Lassman, Jeffrey R. Pierce, Evelyn J. Bangs, Amy P. Sullivan, Bonne Ford, Gizaw Mengistu Tsidu, James P. Sherman, Jeffrey L. Collett, Solomon Bililign. Using Low-Cost Measurement Systems to Investigate Air Quality: A Case Study in Palapye, Botswana. Atmosphere 2020, 11 (6) , 583. https://doi.org/10.3390/atmos11060583
  15. Erin E. McDuffie, Steven J. Smith, Patrick O'Rourke, Kushal Tibrewal, Chandra Venkataraman, Eloise A. Marais, Bo Zheng, Monica Crippa, Michael Brauer, Randall V. Martin. A global anthropogenic emission inventory of atmospheric pollutants from sector- and fuel-specific sources (1970–2017): an application of the Community Emissions Data System (CEDS). Earth System Science Data 2020, 12 (4) , 3413-3442. https://doi.org/10.5194/essd-12-3413-2020

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