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Self-Probing Spectroscopy of the SF6 Molecule: A Study of the Spectral Amplitude and Phase of the High Harmonic Emission

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Download Hi-Res ImageDownload to MS-PowerPointCite This:J. Phys. Chem. A 2015, 119, 23, 6111-6122
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    Self-Probing Spectroscopy of the SF6 Molecule: A Study of the Spectral Amplitude and Phase of the High Harmonic Emission
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    † Laboratoire Interactions, Dynamique et Lasers, IRAMIS, CEA-Saclay, 91191 Gif-sur-Yvette, France
    ‡ Laboratoire de Chimie Physique-Matière et Rayonnement, UMR 7614, UPMC Univ. Paris 06, 11 Rue Pierre et Marie Curie, 75231 Paris Cedex 05, France
    § Department of Physics, Lund University, P.O. Box 118, SE-22100 Lund, Sweden
    ∥ Laboratorium für Physikalische Chemie, ETH Zürich, Wolfgang-Pauli-Strasse 10, 8093 Zürich, Switzerland
    ⊥ Helmholtz-Institute-Jena, Fröbelstieg 3, 07743 Jena, Germany
    # Department of Physics, The Ohio State University, Columbus, Ohio 43210, United States
    *B. Manschwetus. E-mail: [email protected]
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    The Journal of Physical Chemistry A

    Cite this: J. Phys. Chem. A 2015, 119, 23, 6111–6122
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    https://doi.org/10.1021/acs.jpca.5b00446
    Published March 26, 2015
    Copyright © 2015 American Chemical Society
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    Abstract

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    We present characterizations of the attosecond pulse train produced in the high harmonic generation (HHG) from SF6 molecules irradiated by a strong pulsed laser field at 800 nm. At harmonic order 17, we observe a minimum in the amplitude of the emitted spectrum and a corresponding distortion in the phase. Our experimental results are compared to two models: a multicenter interference model focused on the effect of the structure of the SF6 molecule in HHG and a model focused on the interferences between multiple ionization channels in HHG. We find that the experimental results agree very well with the multiple ionization channels model, illustrating that HHG in molecules can be very complex and that it provides insights of the intramolecular electron dynamics during the interaction process.

    Copyright © 2015 American Chemical Society

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    Cited By

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    This article is cited by 9 publications.

    1. Etienne Plésiat, Sophie E. Canton, John D. Bozek, Piero Decleva, Fernando Martín. Resonant Photoelectron Confinement in the SF6 Molecule. The Journal of Physical Chemistry A 2019, 123 (5) , 1062-1068. https://doi.org/10.1021/acs.jpca.8b12237
    2. Xu-Cong Zhou, Shang Shi, Fei Li, Ying-Chun Guo, Yu-Jun Yang, Qing-Tian Meng, Jing Chen, Xiao-Jun Liu, Bingbing Wang. The interference fringes of above-threshold ionization spectrum of SF 6 molecules in an IR + XUV laser field. Journal of Physics B: Atomic, Molecular and Optical Physics 2020, 53 (19) , 195101. https://doi.org/10.1088/1361-6455/aba4c5
    3. R. Klas, A. Kirsche, M. Tschernajew, J. Rothhardt, J. Limpert. Annular beam driven high harmonic generation for high flux coherent XUV and soft X-ray radiation. Optics Express 2018, 26 (15) , 19318. https://doi.org/10.1364/OE.26.019318
    4. M. Monfared, E. Irani, R. Sadighi-Bonabi. Controlling the multi-electron dynamics in the high harmonic spectrum from N2O molecule using TDDFT. The Journal of Chemical Physics 2018, 148 (23) https://doi.org/10.1063/1.5025155
    5. D. D. A. Clarke, H. W. van der Hart, A. C. Brown. Extreme-ultraviolet-initiated high-order harmonic generation in Ar + . Physical Review A 2018, 97 (2) https://doi.org/10.1103/PhysRevA.97.023413
    6. Gal Orenstein, Oren Pedatzur, Ayelet J. Uzan, Barry D. Bruner, Yann Mairesse, Nirit Dudovich. Isolating strong-field dynamics in molecular systems. Physical Review A 2017, 95 (5) https://doi.org/10.1103/PhysRevA.95.051401
    7. B. P. Wilson, K. D. Fulfer, S. Mondal, X. Ren, J. Tross, E. D. Poliakoff, J. Jose, Anh-Thu Le, R. R. Lucchese, C. Trallero-Herrero. High order harmonic generation from SF6: Deconvolution of macroscopic effects. The Journal of Chemical Physics 2016, 145 (22) https://doi.org/10.1063/1.4971244
    8. S. Odžak, E. Hasović, D. B. Milošević. High-order harmonic generation in polyatomic molecules induced by a bicircular laser field. Physical Review A 2016, 94 (3) https://doi.org/10.1103/PhysRevA.94.033419
    9. K. Veyrinas, V. Gruson, S. J. Weber, L. Barreau, T. Ruchon, J.-F. Hergott, J.-C. Houver, R. R. Lucchese, P. Salières, D. Dowek. Molecular frame photoemission by a comb of elliptical high-order harmonics: a sensitive probe of both photodynamics and harmonic complete polarization state. Faraday Discussions 2016, 194 , 161-183. https://doi.org/10.1039/C6FD00137H
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    The Journal of Physical Chemistry A

    Cite this: J. Phys. Chem. A 2015, 119, 23, 6111–6122
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.jpca.5b00446
    Published March 26, 2015
    Copyright © 2015 American Chemical Society
    Request reuse permissions

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