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Experimental Evidence of a Stable 2H Phase on the Surface of Layered 1T′-TaTe2

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Download Hi-Res ImageDownload to MS-PowerPointCite This:J. Phys. Chem. C 2021, 125, 1, 1150-1156
    C: Physical Properties of Materials and Interfaces

    Experimental Evidence of a Stable 2H Phase on the Surface of Layered 1T′-TaTe2
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    • Indrani Kar
      Indrani Kar
      Department of Condensed Matter Physics and Material Sciences, S N Bose National Centre for Basic Sciences, Kolkata, West Bengal 700106, India
      More by Indrani Kar
    • Kapildeb Dolui
      Kapildeb Dolui
      Department of Physics and Astronomy, University of Delaware, Newark, Delaware 19716-5600, United States
      More by Kapildeb Dolui
    • Luminita Harnagea
      Luminita Harnagea
      Indian Institute of Science Education and Research, Dr. Homi Bhabha Road, Pune, Maharashtra 411008, India
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    • Yevhen Kushnirenko
      Yevhen Kushnirenko
      Leibniz-Institute for Solid State and Materials Research Dresden, P.O.Box 270116, D-01171, Dresden 01069, Germany
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    • Grigory Shipunov
      Grigory Shipunov
      Leibniz-Institute for Solid State and Materials Research Dresden, P.O.Box 270116, D-01171, Dresden 01069, Germany
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    • Nicholas C. Plumb
      Nicholas C. Plumb
      Swiss Light Source, Paul Scherrer Institute, Villigen PSI CH-5232, Switzerland
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    • Ming Shi
      Ming Shi
      Swiss Light Source, Paul Scherrer Institute, Villigen PSI CH-5232, Switzerland
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    • Bernd Büchner
      Bernd Büchner
      Leibniz-Institute for Solid State and Materials Research Dresden, P.O.Box 270116, D-01171, Dresden 01069, Germany
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    • Setti Thirupathaiah*
      Setti Thirupathaiah
      Department of Condensed Matter Physics and Material Sciences, S N Bose National Centre for Basic Sciences, Kolkata, West Bengal 700106, India
      *Email: [email protected]
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      Orcidhttp://orcid.org/0000-0003-1258-0981
    Other Access OptionsSupporting Information (1)

    The Journal of Physical Chemistry C

    Cite this: J. Phys. Chem. C 2021, 125, 1, 1150–1156
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.jpcc.0c10517
    Published January 2, 2021
    Copyright © 2021 American Chemical Society
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    Abstract

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    We report on the low-energy electronic structure of tantalum ditelluride (1T′-TaTe2), one of the charge density wave (CDW) materials from the group V transition metal dichalcogenides using angle-resolved photoemission spectroscopy and density functional theory (DFT). We find that the Fermi surface topology of TaTe2 is quite complicated compared to its isovalent compounds such as TaS2, TaSe2, and isostructural compound NbTe2. Most importantly, we discover that the surface electronic structure of 1T′-TaTe2 has more resemblance to the 2H-TaTe2, while the bulk electronic structure has more resemblance to the hypothetical 1T-TaTe2. These experimental observations are thoroughly compared with our DFT calculations performed on 1T-, 2H-, and 2H (monolayer)/1T-TaTe2. We further notice that the Fermi surface topology is temperature independent up to 180 K, confirming that the 2H phase on the surface is stable up to 180 K and the CDW order is not due to the Fermi surface nesting.

    Copyright © 2021 American Chemical Society

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    Supporting Information

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    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acs.jpcc.0c10517.

    • EDX measurements, additional ARPES data, and bulk DFT calculations of TaTe2 in 1T and 2H phases (PDF)

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    Cited By

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    This article is cited by 11 publications.

    1. Tong Su, Huizhen Li, Gan Liu, Jianling Liang, Jian Shao, Haipeng Zhu, Kang Li, Xiaoxiang Xi, Weiwei Zhao. Electrostatic Doping of Electron–Phonon Interaction in 1T′-TaTe2 with an Electric Double Layer Interface. The Journal of Physical Chemistry C 2024, 128 (15) , 6412-6418. https://doi.org/10.1021/acs.jpcc.3c08010
    2. Scott Stonemeyer, Mehmet Dogan, Jeffrey D. Cain, Amin Azizi, Derek C. Popple, Austin Culp, Chengyu Song, Peter Ercius, Marvin L. Cohen, Alex Zettl. Targeting One- and Two-Dimensional Ta–Te Structures via Nanotube Encapsulation. Nano Letters 2022, 22 (6) , 2285-2292. https://doi.org/10.1021/acs.nanolett.1c04615
    3. Till Domröse, Claus Ropers. Femtosecond trimer quench in the unconventional charge-density-wave material 1 T ′ − TaTe 2 . Physical Review B 2024, 110 (8) https://doi.org/10.1103/PhysRevB.110.085155
    4. Natsuki Mitsuishi, Yusuke Sugita, Tomoki Akiba, Yuki Takahashi, Masato Sakano, Koji Horiba, Hiroshi Kumigashira, Hidefumi Takahashi, Shintaro Ishiwata, Yukitoshi Motome, Kyoko Ishizaka. Unveiling the orbital-selective electronic band reconstruction through the structural phase transition in TaTe 2 . Physical Review Research 2024, 6 (1) https://doi.org/10.1103/PhysRevResearch.6.013155
    5. Jong Hun Kim, Hayeong Sung, Gwan-Hyoung Lee. Phase Engineering of Two‐Dimensional Transition Metal Dichalcogenides. Small Science 2024, 4 (1) https://doi.org/10.1002/smsc.202300093
    6. Kang-Jun Lu, Yi-Fan Wang, Qian Xia, Gui-Tao Zhang, Qian Chen, . Structural phase transition induced enhancement of carrier mobility of monolayer RuSe<sub>2</sub>. Acta Physica Sinica 2024, 73 (14) , 146302. https://doi.org/10.7498/aps.73.20240557
    7. Sandeep kumar, Surender Pratap, Nikunj Joshi, Ravi Trivedi, Chandra Sekhar Rout, Brahmananda Chakraborty. Recent development of two-dimensional tantalum dichalcogenides and their applications. Micro and Nanostructures 2023, 181 , 207627. https://doi.org/10.1016/j.micrna.2023.207627
    8. Iolanda Di Bernardo, Joan Ripoll‐Sau, Jose Angel Silva‐Guillén, Fabian Calleja, Cosme G. Ayani, Rodolfo Miranda, Enric Canadell, Manuela Garnica, Amadeo L. Vázquez de Parga. Metastable Polymorphic Phases in Monolayer TaTe 2. Small 2023, 19 (29) https://doi.org/10.1002/smll.202300262
    9. Yi Lin, Maximillian Huber, Sangeeta Rajpurohit, Yanglin Zhu, Khalid M. Siddiqui, Daniel H. Eilbott, Luca Moreschini, Ping Ai, Jonathan D. Denlinger, Zhiqiang Mao, Liang Z. Tan, Alessandra Lanzara. Evidence of nested quasi-one-dimensional Fermi surface and decoupled charge-lattice orders in layered TaTe 2 . Physical Review Research 2022, 4 (2) https://doi.org/10.1103/PhysRevResearch.4.L022009
    10. Nashra Pistawala, Dibyata Rout, Kumar Saurabh, Rabindranath Bag, Koushik Karmakar, Luminita Harnagea, Surjeet Singh. Crystal growth of quantum materials: a review of selective materials and techniques. Bulletin of Materials Science 2022, 45 (1) https://doi.org/10.1007/s12034-021-02612-1
    11. T. C. Hu, Q. Wu, Z. X. Wang, L. Y. Shi, Q. M. Liu, L. Yue, S. J. Zhang, R. S. Li, X. Y. Zhou, S. X. Xu, D. Wu, T. Dong, N. L. Wang. Optical spectroscopy and ultrafast pump-probe study of the structural phase transition in 1 T ′ − TaTe 2 . Physical Review B 2022, 105 (7) https://doi.org/10.1103/PhysRevB.105.075113
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    The Journal of Physical Chemistry C

    Cite this: J. Phys. Chem. C 2021, 125, 1, 1150–1156
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.jpcc.0c10517
    Published January 2, 2021
    Copyright © 2021 American Chemical Society
    Request reuse permissions

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