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Heterogeneous Nucleation onto Ions and Neutralized Ions: Insights into Sign-Preference

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    Heterogeneous Nucleation onto Ions and Neutralized Ions: Insights into Sign-Preference
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    † Department of Physics, University of Helsinki, P.O. Box 64, 00014 Helsinki, Finland
    ‡ University Paris Est Creteil, University Paris-Diderot, LISA, UMR CNRS 7583, Paris, France
    § Department of Chemistry, University of Helsinki, P.O. Box 55, 00014 Helsinki, Finland
    ∥ Aerodyne Research Inc., Billerica, Massachusetts, United States
    ⊥ Paul Scherrer Institut, 5232 Villigen PSI, Switzerland
    *Phone +358503185096. E-mail: [email protected]
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    The Journal of Physical Chemistry C

    Cite this: J. Phys. Chem. C 2016, 120, 13, 7444–7450
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    https://doi.org/10.1021/acs.jpcc.6b01779
    Published March 15, 2016
    Copyright © 2016 American Chemical Society
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    Abstract

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    Heterogeneous nucleation of vapor on a seed particle surface is dependent on the seed properties such as size, chemical composition, and electric charging state, of which the significance of the charging state has not been uncovered unambiguously. The underlying problem is that, on the molecular level, the charging state and the chemical composition of the seed are connected and cannot be well separated without a direct mass spectrometric measurement of the ion. By generating sub-3 nm size selected seeds of different size, chemical composition, electric charging state, and letting three different vapors nucleate onto the seeds, we show that heterogeneous nucleation does not clearly prefer either positive or negative seeds. Rather, the most important parameter determining the nucleation probability in the sub-3 nm size range was the seed chemical composition. Our findings help to understand the dynamics in various nanoparticle systems, such as nucleation chambers, industrial processes, or atmospheric aerosols.

    Copyright © 2016 American Chemical Society

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    This article is cited by 42 publications.

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    Cite this: J. Phys. Chem. C 2016, 120, 13, 7444–7450
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.jpcc.6b01779
    Published March 15, 2016
    Copyright © 2016 American Chemical Society
    Request reuse permissions

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