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Colloidal Particles in Thin Nematic Wetting Films

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Université de Tunis El Manar, Faculté des Sciences de Tunis, LR99ES16 Laboratoire Physique de la Matière Molle et de la Modélisation Electromagnétique, 2092, Tunis, Tunisia
Max-Planck-Institut für Intelligente Systeme, Heisenbergstraße 3, D-70569 Stuttgart, Germany
§ Institut für Theoretische Physik IV, Universität Stuttgart, Pfaffenwaldring 57, D-70569 Stuttgart, Germany
Laboratoire Charles Coulomb, UMR 5221, CNRS-Université de Montpellier, 34095 Montpellier, France
Cite this: Langmuir 2016, 32, 35, 9097–9107
Publication Date (Web):August 18, 2016
https://doi.org/10.1021/acs.langmuir.6b02701
Copyright © 2016 American Chemical Society
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Abstract

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We experimentally and theoretically study the variety of elastic deformations that appear when colloidal inclusions are embedded in thin wetting films of a nematic liquid crystal with hybrid anchoring conditions. In the thickest films, the elastic dipoles formed by particles and their accompanying defects share features with the patterns commonly observed in liquid crystal cells. When the film gets thinner than the particles size, however, the capillary effects strongly modify the appearance of the elastic dipoles and the birefringence patterns. The influence of the film thickness and particles sizes on the patterns has been explored. The main experimental features and the transitions observed at large scale—with respect to the inclusions’ size—are explained with a simple two-dimensional Ansatz, combining capillarity and nematic elasticity. In a second step, we discuss the origin of the variety of observed textures. Developing a three-dimensional Landau-de Gennes model at the scale of the particles, we show that the presence of free interfaces and the beads confinement yield metastable configurations that are quenched during the film spreading or the beads trapping at interfaces.

Cited By


This article is cited by 2 publications.

  1. Mohamed Amine Gharbi, Daniel A. Beller, Nima Sharifi-Mood, Rohini Gupta, Randall D. Kamien, Shu Yang, and Kathleen J. Stebe . Elastocapillary Driven Assembly of Particles at Free-Standing Smectic-A Films. Langmuir 2018, 34 (5) , 2006-2013. https://doi.org/10.1021/acs.langmuir.7b03351
  2. Hao Qiao, Shasha Feng, Ze-xian Low, Jiarui Chen, Feng Zhang, Zhaoxiang Zhong, Weihong Xing. Al-DTPA microfiber assisted formwork construction technology for high-performance SiC membrane preparation. Journal of Membrane Science 2020, 594 , 117464. https://doi.org/10.1016/j.memsci.2019.117464

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