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Single-Material Organic Solar Cells Based on Electrospun Fullerene-Grafted Polythiophene Nanofibers

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Download Hi-Res ImageDownload to MS-PowerPointCite This:Macromolecules 2017, 50, 13, 4972-4981
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    Single-Material Organic Solar Cells Based on Electrospun Fullerene-Grafted Polythiophene Nanofibers
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    † †Department of Biosystems and Soft Matter, Institute of Fundamental Technological Research, and ‡Laboratory of Polymers and Biomaterials, Institute of Fundamental Technological Research, Polish Academy of Sciences, Warsaw 02-106, Poland
    § Department of Industrial Chemistry “Toso Montanari”, Alma Mater Studiorum University of Bologna, Bologna 40136, Italy
    *E-mail: [email protected] (F.P.).
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    Macromolecules

    Cite this: Macromolecules 2017, 50, 13, 4972–4981
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    https://doi.org/10.1021/acs.macromol.7b00857
    Published June 28, 2017
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    Abstract

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    Highly efficient single-material organic solar cells (SMOCs) based on fullerene-grafted polythiophenes were fabricated by incorporating electrospun one-dimensional (1D) nanostructures obtained from polymer chain stretching. Poly(3-alkylthiophene) chains were chemically tailored in order to reduce the side effects of charge recombination which severely affected SMOC photovoltaic performance. This enabled us to synthesize a donor–acceptor conjugated copolymer with high solubility, molecular weight, regioregularity, and fullerene content. We investigated the correlations among the active layer hierarchical structure given by the inclusion of electrospun nanofibers and the solar cell photovoltaic properties. The results indicated that SMOC efficiency can be strongly increased by optimizing the supramolecular and nanoscale structure of the active layer, while achieving the highest reported efficiency value (PCE = 5.58%). The enhanced performance may be attributed to well-packed and properly oriented polymer chains. Overall, our work demonstrates that the active material structure optimization obtained by including electrospun nanofibers plays a pivotal role in the development of efficient SMOCs and suggests an interesting perspective for the improvement of copolymer-based photovoltaic device performance using an alternative pathway.

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    The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acs.macromol.7b00857.

    • 1H NMR spectrum of PRE; 1H NMR spectrum of CoP(3DDT)-(C60HT); FT-IR spectra of PRE and CoP(3DDT)-(C60HT); FT-IR absorption bands and signal assignments for PRE and CoP(3DDT)-(C60HT); GPC trace of CoP(3DDT)-(C60HT); TGA curves of the electrospun nanofibers before and after postproduction treatment; summary of photovoltaic response data of the BHJ reference cell and different SMOCs; SMOCs efficiency as a function of device storage time (PDF)

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    This article is cited by 114 publications.

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    Cite this: Macromolecules 2017, 50, 13, 4972–4981
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    https://doi.org/10.1021/acs.macromol.7b00857
    Published June 28, 2017
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