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Long-Range Dipole–Dipole Interactions in a Plasmonic Lattice

  • Ashwin K. Boddeti
    Ashwin K. Boddeti
    Elmore Family School of Electrical and Computer Engineering, Birck Nanotechnology Center, Purdue University, West Lafayette, Indiana 47907, United States
  • Jun Guan
    Jun Guan
    Department of Chemistry, Northwestern University, Evanston, Illinois 60208, United States
    More by Jun Guan
  • Tyler Sentz
    Tyler Sentz
    Elmore Family School of Electrical and Computer Engineering, Birck Nanotechnology Center, Purdue University, West Lafayette, Indiana 47907, United States
    More by Tyler Sentz
  • Xitlali Juarez
    Xitlali Juarez
    Department of Materials Science and Engineering, Northwestern University, Evanston, Illinois 60208, United States
  • Ward Newman
    Ward Newman
    Intel Corporation, Hillsboro, Oregon 97124, United States
    More by Ward Newman
  • Cristian Cortes
    Cristian Cortes
    Center for Nanoscale Materials, Argonne National Laboratory, Lemont, Illinois 60439, United States
  • Teri W. Odom
    Teri W. Odom
    Department of Chemistry, and Department of Materials Science and Engineering, Northwestern University, Evanston, Illinois 60208, United States
    More by Teri W. Odom
  • , and 
  • Zubin Jacob*
    Zubin Jacob
    Elmore Family School of Electrical and Computer Engineering, Birck Nanotechnology Center, Purdue University, West Lafayette, Indiana 47907, United States
    *Email: [email protected]
    More by Zubin Jacob
Cite this: Nano Lett. 2022, 22, 1, 22–28
Publication Date (Web):October 21, 2021
https://doi.org/10.1021/acs.nanolett.1c02835
Copyright © 2021 American Chemical Society

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    Abstract

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    Spontaneous emission of quantum emitters can be enhanced by increasing the local density of optical states, whereas engineering dipole–dipole interactions requires modifying the two-point spectral density function. Here, we experimentally demonstrate long-range dipole–dipole interactions (DDIs) mediated by surface lattice resonances in a plasmonic nanoparticle lattice. Using angle-resolved spectral measurements and fluorescence lifetime studies, we show that unique nanophotonic modes mediate long-range DDI between donor and acceptor molecules. We observe significant and persistent DDI strengths for a range of densities that map to ∼800 nm mean nearest-neighbor separation distance between donor and acceptor dipoles, a factor of ∼100 larger than free space. Our results pave the way to engineer and control long-range DDIs between an ensemble of emitters at room temperature.

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    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acs.nanolett.1c02835.

    • Numerical simulations including angle-resolved extinction and computing the dyadic Green function; experimental setup; sample fabrication; polymer thin-film thickness; mean nearest-neighbor separation between donor–acceptor pairs; persistence of interactions; and mean decay rate statistics (PDF)

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