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Highly Crystalline Layered VS2 Nanosheets for All-Solid-State Lithium Batteries with Enhanced Electrochemical Performances

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    Research Article

    Highly Crystalline Layered VS2 Nanosheets for All-Solid-State Lithium Batteries with Enhanced Electrochemical Performances
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    • Liangting Cai
      Liangting Cai
      College of Materials and Chemical Engineering, China Three Gorges University, 8 Daxue Road, Yichang, Hubei 443002, P. R. China
      Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, Zhejiang 315201, P. R. China
      More by Liangting Cai
    • Qiang Zhang
      Qiang Zhang
      Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, Zhejiang 315201, P. R. China
      University of Chinese Academy of Sciences, Beijing 100049, P. R. China
      More by Qiang Zhang
    • Jean Pierre Mwizerwa
      Jean Pierre Mwizerwa
      Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, Zhejiang 315201, P. R. China
      University of Chinese Academy of Sciences, Beijing 100049, P. R. China
      More by Jean Pierre Mwizerwa
    • Hongli Wan
      Hongli Wan
      Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, Zhejiang 315201, P. R. China
      University of Chinese Academy of Sciences, Beijing 100049, P. R. China
      More by Hongli Wan
    • Xuelin Yang*
      Xuelin Yang
      College of Materials and Chemical Engineering, China Three Gorges University, 8 Daxue Road, Yichang, Hubei 443002, P. R. China
      *E-mail: [email protected] (X.L.Y.).
      More by Xuelin Yang
      Orcidhttp://orcid.org/0000-0001-5626-701X
    • Xiaoxiong Xu
      Xiaoxiong Xu
      Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, Zhejiang 315201, P. R. China
      More by Xiaoxiong Xu
      Orcidhttp://orcid.org/0000-0002-8599-4918
    • Xiayin Yao*
      Xiayin Yao
      Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, Zhejiang 315201, P. R. China
      *E-mail: [email protected] (X.Y.Y.).
      More by Xiayin Yao
      Orcidhttp://orcid.org/0000-0002-2224-4247
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    ACS Applied Materials & Interfaces

    Cite this: ACS Appl. Mater. Interfaces 2018, 10, 12, 10053–10063
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    https://doi.org/10.1021/acsami.7b18798
    Published March 2, 2018
    Copyright © 2018 American Chemical Society
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    All-solid-state lithium batteries employing inorganic solid electrolytes have been regarded as an ultimate solution to safety issues because of their features of no leakage as well as incombustibility and they are expected to achieve higher energy densities owing to their simplified structure. Two-dimensional transition-metal dichalcogenides exhibit a great potential in energy storage devices because of their unique physical and chemical characteristics. In this work, 50 nm thick highly crystalline layered VS2 (hc-VS2) nanosheets are prepared by a solvothermal method, and their electrochemical performances are evaluated in Li/75% Li2S-24% P2S5-1% P2O5/Li10GeP2S12/hc-VS2 all-solid-state lithium batteries. At 50 mA g–1, hc-VS2 nanosheets show a high reversible capacity of 532.2 mAh g–1 after 30 cycles. Moreover, stable discharge capacities are maintained at 436.8 and 270.4 mAh g–1 at 100 and 500 mA g–1 after 100 cycles, respectively. The superior rate capability and cycling stability are ascribed to the better electronic conductivity and well-developed layered structure. In addition, the electrochemical reaction kinetics and capacity contributions were analyzed via cyclic voltammetry measurements at different scan rates.

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    Cite this: ACS Appl. Mater. Interfaces 2018, 10, 12, 10053–10063
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