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Aqueous Mg-Ion Battery Based on Polyimide Anode and Prussian Blue Cathode

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† Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Institute of New Energy, iChEM(Collaborative Innovation Center of Chemistry for Energy Materials), Fudan University, Shanghai 200433, China
‡ Department of Chemistry, Chemical Theory Center, and Minnesota Supercomputing Institute, University of Minnesota, 207 Pleasant Street SE, Minneapolis, Minnesota 55455-0431, United States
§ Department of Chemical and Biomolecular Engineering, University of Maryland, College Park, Maryland 20742, United States
*E-mail: [email protected]
*E-mail: [email protected]
Cite this: ACS Energy Lett. 2017, 2, 5, 1115–1121
Publication Date (Web):April 18, 2017
https://doi.org/10.1021/acsenergylett.7b00040
Copyright © 2017 American Chemical Society
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    Abstract

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    The magnesium-metal battery, which consists of a cathode, a Mg-metal anode, and a nonaqueous electrolyte, is a safer and less expensive alternative to the popular Li-ion battery. However, the performance of Mg batteries is greatly limited by the low electrochemical oxidative stability of nonaqueous electrolytes, the slow Mg2+ diffusion into the cathode, and the irreversibility of Mg striping and plating on the Mg metal anode. Here, we report the first Mg-ion battery using a Mg2+ aqueous electrolyte, nickel hexacyanoferrate cathode, and polyimide anode. The operation depends on Mg2+ intercalation–deintercalation at the cathode and reversible enolization at the anode, accompanied by Mg2+ transport between cathode and anode. The cell exhibits a maximum cell voltage of 1.5 V and a supercapacitor-like high power, and it can be cycled 5000 times. This system points the way to improved Mg-based rechargeable batteries.

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