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Advancing SPRi Measurements with Novel Biosensors for Studying Surface-Biomolecule Interactions

  • Michael C. Weiger*
    Michael C. Weiger
    Polymers Division, National Institute of Standards and Technology, Gaithersburg, MD 20899
    New Jersey Center for Biomaterials, Rutgers University, Piscataway, NJ 08854
    Department of Polymer Science, University of Akron, Akron, OH 44325
    *[email protected]
  • Khaled Aamer
    Khaled Aamer
    Polymers Division, National Institute of Standards and Technology, Gaithersburg, MD 20899
    New Jersey Center for Biomaterials, Rutgers University, Piscataway, NJ 08854
    Department of Polymer Science, University of Akron, Akron, OH 44325
    More by Khaled Aamer
  • Joachim Kohn
    Joachim Kohn
    Polymers Division, National Institute of Standards and Technology, Gaithersburg, MD 20899
    New Jersey Center for Biomaterials, Rutgers University, Piscataway, NJ 08854
    Department of Polymer Science, University of Akron, Akron, OH 44325
    More by Joachim Kohn
  • , and 
  • Matthew L. Becker
    Matthew L. Becker
    Polymers Division, National Institute of Standards and Technology, Gaithersburg, MD 20899
    New Jersey Center for Biomaterials, Rutgers University, Piscataway, NJ 08854
    Department of Polymer Science, University of Akron, Akron, OH 44325
DOI: 10.1021/bk-2010-1054.ch005
    Publication Date (Web):November 18, 2010
    Copyright © 2010 American Chemical Society
    Biomaterials
    Chapter 5pp 109-124
    ACS Symposium SeriesVol. 1054
    ISBN13: 9780841225671eISBN: 9780841225688

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    Abstract

    Through years of scientific research and development, surface plasmon resonance (SPR) has become a sensitive, quantitative and rapid measurement method with abundant applications in the fields of biology and biomaterials. The present contribution provides a brief overview of SPR history, development of SPR imaging and expanding sensor platforms while also briefly reviewing their many applications. We supplement these discussions with the introduction of new biosensor platforms for SPR imaging 1) composed of the primary mineral component in bone, hydroxyapatite (HA) and 2) tyrosine-derived polycarbonates which are utilized in many biomedical applications. These biosensors are completed with microfluidic flow channels to facilitate kinetic measurements. We describe the fabrication of the multilayer sensor surfaces and also demonstrate surface plasmon generation. We also highlight the utility and potential of these sensor platforms to characterize the binding kinetics of small peptides, engineered to bind specifically to these materials in order to facilitate development of new probes and modifiers for biomaterials.

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