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Combinatorial Pulsed Laser Deposition of Magnetic and Magneto-optical Sr(GaxTiyFe0.34–0.40)O3−δ Perovskite Films

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    Research Article

    Combinatorial Pulsed Laser Deposition of Magnetic and Magneto-optical Sr(GaxTiyFe0.34–0.40)O3−δ Perovskite Films
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    † Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, United States
    ‡ School of Materials Science and Engineering, Harbin Institute of Technology, Harbin 150001, People’s Republic of China
    § Singapore-MIT Alliance, National University of Singapore, 4 Engineering Drive 3, Singapore 117576
    *E-mail: [email protected]
    *E-mail: [email protected]
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    ACS Combinatorial Science

    Cite this: ACS Comb. Sci. 2014, 16, 11, 640–646
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    https://doi.org/10.1021/co5000773
    Published October 8, 2014
    Copyright © 2014 American Chemical Society
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    Abstract

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    Ferromagnetic Sr(GaxTiyFe0.34–0.40)O3−δ (0.1 ≤ x, y ≤ 0.5) films with single-crystal perovskite structure were epitaxially grown on (001) (LaAlO3)0.3(Sr2AlTaO6)0.7 substrates by combinatorial pulsed laser deposition (CPLD) and compared with previous results from films grown from single targets. In CPLD films the Fe was present as both Fe2+ and Fe3+. The distribution of Sr, Ga, Ti, and O was homogeneous, but Fe-rich nanowires with diameter of 3 nm were present perpendicular to the film plane. The unit cell was tetragonally distorted with the ratio of out-of-plane to in-plane lattice parameter decreasing from 1.06 to 1.02 as the Ga content increased. The magnetic easy axis of the films changed from out-of-plane when Ti content y > 0.3 to isotropic as the Ga content increased, consistent with a reduction in magnetoelastic anisotropy. The Ga lowered the Faraday rotation and the magnetization but increased the optical transmittance.

    Copyright © 2014 American Chemical Society

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    Cited By

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    This article is cited by 9 publications.

    1. Paul F. Newhouse, Lan Zhou, Mitsutaro Umehara, David A. Boyd, Edwin Soedarmadji, Joel A. Haber, John M. Gregoire. Bi Alloying into Rare Earth Double Perovskites Enhances Synthesizability and Visible Light Absorption. ACS Combinatorial Science 2020, 22 (12) , 895-901. https://doi.org/10.1021/acscombsci.0c00177
    2. Harrison Sejoon Kim, Joy S. Lee, Si Joon Kim, Jaebeom Lee, Antonio T. Lucero, Myung Mo Sung, Jiyoung Kim. Realization of Spatially Addressable Library by a Novel Combinatorial Approach on Atomic Layer Deposition: A Case Study of Zinc Oxide. ACS Combinatorial Science 2019, 21 (6) , 445-455. https://doi.org/10.1021/acscombsci.9b00007
    3. Chen Zhang, Dong Hun Kim, Xiaohu Huang, Xue Yin Sun, Nicolas M. Aimon, Soo Jin Chua, and Caroline A. Ross . Magnetic and Photoluminescent Coupling in SrTi0.87Fe0.13O3−δ/ZnO Vertical Nanocomposite Films. ACS Applied Materials & Interfaces 2017, 9 (37) , 32359-32368. https://doi.org/10.1021/acsami.7b08741
    4. Dong Hun Kim, XueYin Sun, Tae Cheol Kim, Yun Jae Eun, Taeho Lee, Sung Gyun Jeong, and Caroline A. Ross . Magnetic Phase Formation in Self-Assembled Epitaxial BiFeO3–MgO and BiFeO3–MgAl2O4 Nanocomposite Films Grown by Combinatorial Pulsed Laser Deposition. ACS Applied Materials & Interfaces 2016, 8 (4) , 2673-2679. https://doi.org/10.1021/acsami.5b10676
    5. E. J. Moon, A. Goyal. Combinatorial synthesis of heteroepitaxial, multi-cation, thin-films via pulsed laser deposition coupled with in-situ, chemical and structural characterization. Scientific Reports 2022, 12 (1) https://doi.org/10.1038/s41598-022-06955-5
    6. Samuel Guerin, Brian E. Hayden. ABO 3 and A 1−x C x B 1−y D y (O 1−z E z ) 3 : review of experimental optimisation of thin film perovskites by high-throughput evaporative physical vapour deposition. Chemical Communications 2019, 55 (68) , 10047-10055. https://doi.org/10.1039/C9CC03518D
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    8. Dong Hun Kim, Junho Yang, Min Seok Kim, Tae Cheol Kim. Structure and magnetic properties of spinel-perovskite nanocomposite thin films on SrTiO 3 (111) substrates. Journal of Crystal Growth 2016, 449 , 62-66. https://doi.org/10.1016/j.jcrysgro.2016.05.041
    9. J. Qiu, G.Z. Liu, J. Wolfman, C. Autret-Lambert, S. Roger, J. Gao. Structure and dielectric characteristics of continuous composition spread Ba1−Sr TiO3 thin films by combinatorial pulsed laser deposition. Ceramics International 2016, 42 (5) , 6408-6412. https://doi.org/10.1016/j.ceramint.2016.01.043
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    ACS Combinatorial Science

    Cite this: ACS Comb. Sci. 2014, 16, 11, 640–646
    Click to copy citationCitation copied!
    https://doi.org/10.1021/co5000773
    Published October 8, 2014
    Copyright © 2014 American Chemical Society
    Request reuse permissions

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