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Comparison of Emissions from Wood Combustion. Part 2: Impact of Combustion Conditions on Emission Factors and Characteristics of Particle-Bound Organic Species and Polycyclic Aromatic Hydrocarbon (PAH)-Related Toxicological Potential

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    Comparison of Emissions from Wood Combustion. Part 2: Impact of Combustion Conditions on Emission Factors and Characteristics of Particle-Bound Organic Species and Polycyclic Aromatic Hydrocarbon (PAH)-Related Toxicological Potential
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    † Department of Sedimentology and Environmental Geology and Interdisciplinary Center for Sustainable Development, Georg-August-University, D-37073 Göttingen, Germany
    ‡ Joint Mass Spectrometry Centre, Cooperation Group “Comprehensive Molecular Analytics”, Helmholtz Zentrum München, D-85764 Neuherberg, Germany
    § Joint Mass Spectrometry Centre, Institute of Chemistry, Division of Analytical and Technical Chemistry, University of Rostock, D-18057 Rostock, Germany
    ∥ Department of Solid Biofuels, Technology and Support Centre (TFZ), D-94315 Straubing, Germany
    *E-mail: [email protected]
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    Energy & Fuels

    Cite this: Energy Fuels 2013, 27, 3, 1482–1491
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    https://doi.org/10.1021/ef301506h
    Published January 31, 2013
    Copyright © 2013 American Chemical Society
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    Abstract

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    The impact of combustion conditions on emission factors and characteristics of log wood combustion was investigated. Two different kinds of log woods (spruce and beech) and one kind of briquette (spruce sawdust) were used to study differences in emission behavior depending upon the wood type. Beech wood was used to examine additionally the impact of different moisture contents and maloperation on emissions of fine particulate matter (PM). Therefore, wood logs with three different levels of moisture content were used. Maloperation was simulated by an overload scenario and an air deficiency scenario. Toxicity equivalent (TEQ) values were calculated for the different combustion conditions. It was found that PM mass varies only by a factor of 8 at a maximum, whereas TEQ values can vary more than a factor of 80 (regular beech wood combustion, 6 μg MJ–1; beech wood combustion in an overloaded combustion chamber, 500 μg MJ–1). In particular, wood with a higher moisture content (19%) released high amounts of intermediate products from lignin and cellulose degradation. The PM emissions in this case were the highest among the tested operation conditions, especially during the initial (cold start) inflaming (660 μg MJ–1), but were not in correspondence with the toxicity potential. The TEQ (37 μg MJ–1) in that case was much lower than during maloperation.

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    Cite this: Energy Fuels 2013, 27, 3, 1482–1491
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    https://doi.org/10.1021/ef301506h
    Published January 31, 2013
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