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One-Dimensional Superlattice Heterostructure Library

  • Yi Li
    Yi Li
    Division of Nanomaterials and Chemistry, Hefei National Laboratory for Physical Sciences at the Microscale, Institute of Energy, Hefei Comprehensive National Science Center, CAS Center for Excellence in Nanoscience, Department of Chemistry, Institute of Biomimetic Materials and Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, University of Science and Technology of China, Hefei, Anhui 230026, China
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  • Chong Zhang
    Chong Zhang
    Division of Nanomaterials and Chemistry, Hefei National Laboratory for Physical Sciences at the Microscale, Institute of Energy, Hefei Comprehensive National Science Center, CAS Center for Excellence in Nanoscience, Department of Chemistry, Institute of Biomimetic Materials and Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, University of Science and Technology of China, Hefei, Anhui 230026, China
    More by Chong Zhang
  • Tao-Tao Zhuang
    Tao-Tao Zhuang
    Division of Nanomaterials and Chemistry, Hefei National Laboratory for Physical Sciences at the Microscale, Institute of Energy, Hefei Comprehensive National Science Center, CAS Center for Excellence in Nanoscience, Department of Chemistry, Institute of Biomimetic Materials and Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, University of Science and Technology of China, Hefei, Anhui 230026, China
  • Yue Lin
    Yue Lin
    Division of Nanomaterials and Chemistry, Hefei National Laboratory for Physical Sciences at the Microscale, Institute of Energy, Hefei Comprehensive National Science Center, CAS Center for Excellence in Nanoscience, Department of Chemistry, Institute of Biomimetic Materials and Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, University of Science and Technology of China, Hefei, Anhui 230026, China
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  • Jie Tian
    Jie Tian
    Engineering and Materials Science Experiment Center, University of Science and Technology of China, Hefei, Anhui 230026, China
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  • Xing-Yu Qi
    Xing-Yu Qi
    Division of Nanomaterials and Chemistry, Hefei National Laboratory for Physical Sciences at the Microscale, Institute of Energy, Hefei Comprehensive National Science Center, CAS Center for Excellence in Nanoscience, Department of Chemistry, Institute of Biomimetic Materials and Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, University of Science and Technology of China, Hefei, Anhui 230026, China
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  • Xufeng Li
    Xufeng Li
    Department of Chemistry, Zhejiang University, Hangzhou, Zhejiang 310027, China
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  • Rui Wang
    Rui Wang
    Division of Nanomaterials and Chemistry, Hefei National Laboratory for Physical Sciences at the Microscale, Institute of Energy, Hefei Comprehensive National Science Center, CAS Center for Excellence in Nanoscience, Department of Chemistry, Institute of Biomimetic Materials and Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, University of Science and Technology of China, Hefei, Anhui 230026, China
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  • Liang Wu
    Liang Wu
    Division of Nanomaterials and Chemistry, Hefei National Laboratory for Physical Sciences at the Microscale, Institute of Energy, Hefei Comprehensive National Science Center, CAS Center for Excellence in Nanoscience, Department of Chemistry, Institute of Biomimetic Materials and Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, University of Science and Technology of China, Hefei, Anhui 230026, China
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  • Guo-Qiang Liu
    Guo-Qiang Liu
    Division of Nanomaterials and Chemistry, Hefei National Laboratory for Physical Sciences at the Microscale, Institute of Energy, Hefei Comprehensive National Science Center, CAS Center for Excellence in Nanoscience, Department of Chemistry, Institute of Biomimetic Materials and Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, University of Science and Technology of China, Hefei, Anhui 230026, China
  • Tao Ma
    Tao Ma
    Division of Nanomaterials and Chemistry, Hefei National Laboratory for Physical Sciences at the Microscale, Institute of Energy, Hefei Comprehensive National Science Center, CAS Center for Excellence in Nanoscience, Department of Chemistry, Institute of Biomimetic Materials and Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, University of Science and Technology of China, Hefei, Anhui 230026, China
    More by Tao Ma
  • Zhen He
    Zhen He
    Division of Nanomaterials and Chemistry, Hefei National Laboratory for Physical Sciences at the Microscale, Institute of Energy, Hefei Comprehensive National Science Center, CAS Center for Excellence in Nanoscience, Department of Chemistry, Institute of Biomimetic Materials and Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, University of Science and Technology of China, Hefei, Anhui 230026, China
    More by Zhen He
  • Hao-Bo Sun
    Hao-Bo Sun
    Division of Nanomaterials and Chemistry, Hefei National Laboratory for Physical Sciences at the Microscale, Institute of Energy, Hefei Comprehensive National Science Center, CAS Center for Excellence in Nanoscience, Department of Chemistry, Institute of Biomimetic Materials and Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, University of Science and Technology of China, Hefei, Anhui 230026, China
    More by Hao-Bo Sun
  • Fengjia Fan
    Fengjia Fan
    CAS Key Laboratory of Microscale Magnetic Resonance and Department of Modern Physics, University of Science and Technology of China, Hefei, Anhui 230026, China
    Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui 230026, China
    More by Fengjia Fan
  • Haiming Zhu
    Haiming Zhu
    Department of Chemistry, Zhejiang University, Hangzhou, Zhejiang 310027, China
    More by Haiming Zhu
  • , and 
  • Shu-Hong Yu*
    Shu-Hong Yu
    Division of Nanomaterials and Chemistry, Hefei National Laboratory for Physical Sciences at the Microscale, Institute of Energy, Hefei Comprehensive National Science Center, CAS Center for Excellence in Nanoscience, Department of Chemistry, Institute of Biomimetic Materials and Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, University of Science and Technology of China, Hefei, Anhui 230026, China
    *[email protected]
    More by Shu-Hong Yu
Cite this: J. Am. Chem. Soc. 2021, 143, 18, 7013–7020
Publication Date (Web):April 30, 2021
https://doi.org/10.1021/jacs.1c01514
Copyright © 2021 American Chemical Society

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    Abstract

    Abstract Image

    Axially, epitaxially organizing nano-objects of distinct compositions and structures into superlattice nanowires enables full utilization of sunlight, readily engineered band structures, and tunable geometric parameters to fit carrier transport, thus holding great promise for optoelectronics and solar-to-fuel conversion. To maximize their efficiency, the general and high-precision synthesis of colloidal axial superlattice nanowires (ASLNWs) with programmable compositions and structures is the prerequisite; however, it remains challenging. Here, we report an axial encoding methodology toward the ASLNW library with precise control over their compositions, dimensions, crystal phases, interfaces, and periodicity. Using a predesigned, editable nanoparticle framework that offers the synthetic selectivity, we are able to chemically decouple adjacent sub-objects in ASLNWs and thus craft them in a controlled approach, yielding a library of distinct ASLNWs. We integrate therein plasmonic, metallic, or near-infrared-active chalcogenides, which hold great potential in solar energy conversion. Such synthetic capability enables a performance boost in target applications, as we report order-of-magnitude enhanced photocatalytic hydrogen production rates using optimized ASLNWs compared to corresponding solo objects. Furthermore, it is expected that such unique superlattice nanowires could bring out new phenomena.

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    • Supplementary notes of derivation of concentration evolution equation, calculation of strain and stress, and structural characterizations (PDF)

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    Cited By

    This article is cited by 15 publications.

    1. Qingzhuo Lin, Shudong Liang, Jintao Wang, Rongbin Zhang, Gang Liu, Xuewen Wang. Hierarchically Periodic Macroporous CdS–ZnO Heterojunctions with Multiple Quantum Well-like Band Alignments for Efficient Photocatalytic Hydrogen Evolution without a Cocatalyst. ACS Sustainable Chemistry & Engineering 2023, 11 (7) , 3093-3102. https://doi.org/10.1021/acssuschemeng.2c07255
    2. Yi Li, Zhen-Chao Shao, Chong Zhang, Shu-Hong Yu. Catalyzed Growth for Atomic-Precision Colloidal Chalcogenide Nanowires and Heterostructures: Progress and Perspective. The Journal of Physical Chemistry Letters 2021, 12 (43) , 10695-10705. https://doi.org/10.1021/acs.jpclett.1c02358
    3. Qian Zhang, Shuaiqi Gao, Yingying Guo, Huiyong Wang, Jishi Wei, Xiaofang Su, Hucheng Zhang, Zhimin Liu, Jianji Wang. Designing covalent organic frameworks with Co-O4 atomic sites for efficient CO2 photoreduction. Nature Communications 2023, 14 (1) https://doi.org/10.1038/s41467-023-36779-4
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    5. Dan Xu, Li Zhai, Zhangyan Mu, Chen-Lei Tao, Feiyue Ge, Han Zhang, Mengning Ding, Fang Cheng, Xue-Jun Wu. Versatile synthesis of nano-icosapods via cation exchange for effective photocatalytic conversion of biomass-relevant alcohols. Chemical Science 2023, 14 (37) , 10167-10175. https://doi.org/10.1039/D3SC02493H
    6. Lu Liu, Yalin He, Sixing Yin, Xiaoqing Chang, Jingyu Zhang, Liang Peng, Jialong Li, Yuzhu Ma, Qiulong Wei, Kun Lan, Dongyuan Zhao. Bimodal ordered porous hierarchies from cooperative soft-hard template pairs. Matter 2023, 6 (9) , 3099-3111. https://doi.org/10.1016/j.matt.2023.07.024
    7. Jun Li, Chaofeng Wang, Shuilin Wu, Zhenduo Cui, Yufeng Zheng, Zhaoyang Li, Hui Jiang, Shengli Zhu, Xiangmei Liu. Superlattice Nanofilm on a Touchscreen for Photoexcited Bacteria and Virus Killing by Tuning Electronic Defects in the Heterointerface. Advanced Materials 2023, 35 (22) https://doi.org/10.1002/adma.202300380
    8. Ting Shi Zhang, Bi Xia Yang, Ming Xiong Lin, Zan Yong Zhuang, Yan Yu. Toward Rational Design of Ordered Heterostructures for Energy and Environmental Sustainability: A Review. Advanced Energy and Sustainability Research 2023, 4 (6) https://doi.org/10.1002/aesr.202200204
    9. Limei Wang, Yu Sun, Fuyong Zhang, Jingting Hu, Wentao Hu, Shunji Xie, Yongke Wang, Jun Feng, Yubing Li, Genyuan Wang, Biao Zhang, Haiyan Wang, Qinghong Zhang, Ye Wang. Precisely Constructed Metal Sulfides with Localized Single‐Atom Rhodium for Photocatalytic C−H Activation and Direct Methanol Coupling to Ethylene Glycol. Advanced Materials 2023, 35 (5) https://doi.org/10.1002/adma.202205782
    10. Yi Li, Shu-Hong Yu. One-dimensional semiconducting hierarchical nanostructures. 2023, 202-225. https://doi.org/10.1016/B978-0-12-822425-0.00100-7
    11. Cheng-zhao Jin, Xin-an Yang, Xiao-min Zhai, Shang-Bing Wang, Wang-bing Zhang. ZnO/Sn3O4 amorphous-crystalline heterojunctions for Cr(VI) visible photocatalysis: Simple synthesis with excellent performance. Applied Surface Science 2023, 608 , 155263. https://doi.org/10.1016/j.apsusc.2022.155263
    12. Ruhua Zha, Chao Li, Liu He, Min Zhang. Two-dimensional defective black phosphorus/BiVO4 nanoheterojunctions for molecular nitrogen activation. Journal of Colloid and Interface Science 2022, 628 , 378-388. https://doi.org/10.1016/j.jcis.2022.07.092
    13. Tongming Su, Chengzheng Men, Liuyun Chen, Bingxian Chu, Xuan Luo, Hongbing Ji, Jianhua Chen, Zuzeng Qin. Sulfur Vacancy and Ti 3 C 2 T x Cocatalyst Synergistically Boosting Interfacial Charge Transfer in 2D/2D Ti 3 C 2 T x /ZnIn 2 S 4 Heterostructure for Enhanced Photocatalytic Hydrogen Evolution. Advanced Science 2022, 9 (4) https://doi.org/10.1002/advs.202103715
    14. Jin-Wu Jiang. One-dimensional transition metal dichalcogenide lateral heterostructures. Physical Chemistry Chemical Physics 2021, 23 (48) , 27312-27319. https://doi.org/10.1039/D1CP04850C
    15. Li Zhai, Zijian Li, Hua Zhang. Enriching the library of axial superlattice nanowires. Science China Materials 2021, 64 (10) , 2627-2628. https://doi.org/10.1007/s40843-021-1716-x

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