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Observation of Resonant Quantum Magnetoelectric Effect in a Multiferroic Metal–Organic Framework

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State Key Laboratory of Magnetism, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, PR China
Cite this: J. Am. Chem. Soc. 2016, 138, 3, 782-785
Publication Date (Web):January 8, 2016
https://doi.org/10.1021/jacs.5b12488
Copyright © 2016 American Chemical Society
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Abstract

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A resonant quantum magnetoelectric coupling effect has been demonstrated in the multiferroic metal–organic framework of [(CH3)2NH2]Fe(HCOO)3. This material shows a coexistence of a spin-canted antiferromagnetic order and ferroelectricity as well as clear magnetoelectric coupling below TN ≈ 19 K. In addition, a component of single-ion quantum magnets develops below ∼8 K because of an intrinsic magnetic phase separation. The stair-shaped magnetic hysteresis loop at 2 K signals resonant quantum tunneling of magnetization. Meanwhile, the magnetic field dependence of dielectric permittivity exhibits sharp peaks just at the critical tunneling fields, evidencing the occurrence of resonant quantum magnetoelectric coupling effect. This resonant effect enables a simple electrical detection of quantum tunneling of magnetization.

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The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/jacs.5b12488.

  • Sample synthesis information, X-ray powder and single-crystal diffraction patterns, experimental details, pyroelectric and electric polarization data, and magnetodielectric effect at 15 K. (PDF)

  • Crystallographic information file for Fe-MOF. (CIF)

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Please note: If you switch to a different device, you may be asked to login again with only your ACS ID.

Please note: If you switch to a different device, you may be asked to login again with only your ACS ID.

Please note: If you switch to a different device, you may be asked to login again with only your ACS ID.

OOPS

You have to login with your ACS ID befor you can login with your Mendeley account.

MENDELEY PAIRING EXPIRED
Your Mendeley pairing has expired. Please reconnect

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CONTINUE