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Hydrogen Generation by Laser Irradiation of Carbon Powder in Water

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Department of Material Science and Chemistry, Faculty of Systems Engineering, Wakayama University, Sakaedani 930, Wakayama 640-8510, Japan
*Tel.: +81-73-457-8295. E-mail: [email protected]
Cite this: J. Phys. Chem. C 2013, 117, 36, 18281–18285
Publication Date (Web):August 19, 2013
https://doi.org/10.1021/jp4012558
Copyright © 2013 American Chemical Society

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    Abstract

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    We report the photochemical activity of carbon powder in the generation of hydrogen from water by laser irradiation, without any electrodes and photocatalysts. The gas was obtained by laser irradiation in the VIS-NIR range and was dependent nonlinearly on the laser power density. From a gas component analysis and a repeated irradiation experiment, it was found that the carbon powder was oxidized and acted as a sacrificial reagent in the photochemical hydrogen generation. In addition, a highly carbonized charcoal, known as Bincho-tan, was found to effectively work for the hydrogen generation.

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    Information regarding carbonation degree of Bincho-tan powder; practical usage of Bincho-tan; or retention capacity of hydrogen in several kinds of glasses. This material is available free of charge via the Internet at http://pubs.acs.org.

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