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Ultraviolet Light-Induced Surface-Initiated Atom-Transfer Radical Polymerization

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State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China
*E-mail: [email protected]
Cite this: ACS Macro Lett. 2013, 2, 7, 592–596
Publication Date (Web):June 12, 2013
https://doi.org/10.1021/mz400237w
Copyright © 2013 American Chemical Society
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Abstract

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UV light-induced surface-initiated atom-transfer radical polymerization (ATRP) was reported. This method uses TiO2 nanoparticles as photoactive materials to reduce Cu(II)/L to a Cu(I)/L complex under UV irradiation by a one-electron transfer process for ATRP with multiple usage of monomer solutions. The growth of polymer brushes can be manipulated by either varying the content of photoactive materials or regulating the irradiation intensity, thereby yielding polymer brushes with controllable thickness, composition, and architecture.

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