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    Enhanced Absorption Induced by a Metallic Nanoshell
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    Department of Physical Chemistry and the Lise Meitner Center for Quantum Chemistry, The Hebrew University of Jerusalem, Jerusalem 91904 Israel
    Department of Chemistry and Biochemistry, University of California, Los Angeles, California 90095-1569
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    Nano Letters

    Cite this: Nano Letters 2004, 4, 1, 85–88
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    https://doi.org/10.1021/nl034902k
    Published December 9, 2003
    Copyright © 2004 American Chemical Society
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    Abstract

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    Nanoshells have been previously shown to have tunable absorption frequencies that are dependent on the ratio of their inner and outer radii. Inspired by this, we ask:  can a nanoshell increase the absorption of a small core system embedded within it? A theoretical model is constructed to answer this question. A core, composed of a “jellium” ball of the density of gold is embedded within a jellium nanoshell of nanometric diameter. The shell plasmon frequency is tuned to the core absorption line. A calculation based the time-dependent density functional theory was performed showing a 10 fold increase in core excitation yield.

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    Cite this: Nano Letters 2004, 4, 1, 85–88
    Click to copy citationCitation copied!
    https://doi.org/10.1021/nl034902k
    Published December 9, 2003
    Copyright © 2004 American Chemical Society
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