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    Nanoscale Imaging of Plasmonic Hot Spots and Dark Modes with the Photothermal-Induced Resonance Technique
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    † Center for Nanoscale Science and Technology, National Institute Standards and Technology, Gaithersburg, 100 Bureau Drive, Maryland 20899, United States
    ‡ Institute for Research in Electronics and Applied Physics (IREAP), University of Maryland, College Park, Maryland 20742, United States
    *E-mail: [email protected]
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    Nano Letters

    Cite this: Nano Lett. 2013, 13, 7, 3218–3224
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    https://doi.org/10.1021/nl401284m
    Published June 18, 2013
    Copyright © 2013 American Chemical Society
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    Abstract

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    The collective oscillation of conduction electrons, responsible for the localized surface plasmon resonances, enables engineering nanomaterials by tuning their optical response from the visible to terahertz as a function of nanostructure size, shape, and environment. While theoretical calculations helped tremendously in understanding plasmonic nanomaterials and optimizing their light matter interaction, only a few experimental techniques are available to study these materials with high spatial resolution. In this work, the photothermal-induced resonance (PTIR) technique is applied for the first time to image the dark plasmonic resonance of gold asymmetric split ring resonators (A-SRRs) in the mid-infrared (IR) spectral region with nanoscale resolution. Additionally, the chemically specific PTIR signal is used to map the local absorption enhancement of poly(methyl methacrylate) coated on A-SRRs, revealing hot spots with local enhancement factors up to ≈30 at 100 nm lateral resolution. We argue that PTIR nanoscale characterization will facilitate the engineering and application of plasmonic nanomaterials for mid-IR applications.

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    Supporting Information

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    Additional A-SRRs FTIR spectra, nanofabrication scheme, SEM images, PTIR spectra, and images as referenced in the main text. This material is available free of charge via the Internet at http://pubs.acs.org.

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    Cite this: Nano Lett. 2013, 13, 7, 3218–3224
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    https://doi.org/10.1021/nl401284m
    Published June 18, 2013
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