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    Three-Dimensional Nanoelectrode by Metal Nanowire Nonwoven Clothes
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    † Department of Materials Science and Engineering, Kyoto University, Kyoto 606-8501, Japan
    ‡ Nanoscience and Nanotechnology Research Center, Osaka Prefecture University, Osaka 599-8570, Japan
    *E-mail: [email protected]
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    Nano Letters

    Cite this: Nano Lett. 2014, 14, 4, 1932–1937
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    https://doi.org/10.1021/nl404753e
    Published March 10, 2014
    Copyright © 2014 American Chemical Society
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    Abstract

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    Metal nanowire nonwoven cloth (MNNC) is a metal sheet that has resulted from intertwined metal nanowires 100 nm in diameter with several dozen micrometers of length. Thus, it is a new metallic material having both a flexibility of the metal sheet and a large specific surface area of the nanowires. As an application that utilizes these properties, we propose a high-cyclability electrode for Li storage batteries, in which an active material is deposited or coated on MNNC. The proposed electrode can work without any binders, conductive additives, and current collectors, which might largely improve a practical gravimetric energy density. Huge electrode surfaces provide efficient ion/electron transports, and sufficient interspaces between the respective nanowires accommodate large volume expansions of the active material. To demonstrate these advantages, we have fabricated a NiO-covered nickel nanowire nonwoven cloth (NNNC) by electroless deposition under a magnetic field and annealing in air. The adequately annealed NNNC was shown to be an excellent conversion-type electrode that exhibits a quite high cyclability, 500 mAh/g at 1 C after 300 cycles, compared to that of a composite electrode consisting of NiO nanoparticles. Thus, the present design concept will contribute to a game-changing technology in future lithium ion battery (LIB) electrodes.

    Copyright © 2014 American Chemical Society

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    Detailed fabrication processes of NiO-covered NNNCs. This material is available free of charge via the Internet at http://pubs.acs.org.

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    Cite this: Nano Lett. 2014, 14, 4, 1932–1937
    Click to copy citationCitation copied!
    https://doi.org/10.1021/nl404753e
    Published March 10, 2014
    Copyright © 2014 American Chemical Society
    Request reuse permissions

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