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Capturing the Optical Phase Response of Nanoantennas by Coherent Second-Harmonic Microscopy

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† ICFO−Institut de Ciences Fotoniques, Mediterranean Technology Park, 08860 Castelldefels Barcelona, Spain
‡ ICREA—Institució Catalana de Recerca i Estudis Avançats, 08010 Barcelona, Spain
*E-mail: [email protected]
Cite this: Nano Lett. 2014, 14, 7, 4078–4082
Publication Date (Web):June 13, 2014
https://doi.org/10.1021/nl501588r
Copyright © 2014 American Chemical Society
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    Abstract

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    The ultrafast coherent control of light localization in resonant plasmonic nanostructures is intricately related to the phase response of the involved plasmon resonances. In this work, we exploit the second harmonic signal generated by single optical nanoantennas subject to broadband phase-controlled femtosecond pulses to study and tailor the coherent resonance response. Our results reveal that both the spectral phase and the amplitude components associated with the plasmon resonance of arbitrary individual nanoantennas can be accurately determined.

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    Details on the nanoantennas invesigated, SEM images of the samples, and MIIPS scans on different nanoantennas. This material is available free of charge via the Internet at http://pubs.acs.org.

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