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Progress, Challenges, and Opportunities in Two-Dimensional Materials Beyond Graphene

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† †Department of Chemistry and Biochemistry and ‡Department of Physics, The Ohio State University, Columbus, Ohio 43210, United States
§ Department of Materials Science and Engineering, North Carolina State University, Raleigh, North Carolina 27607, United States
⊥ Department of Materials Science and Engineering, Stanford University, Palo Alto, California 94305, United States
∥ Department of Physics and Electrical Engineering, Columbia University, New York, New York 10027, United States
Department of Materials Science and Engineering, Northwestern University, Evanston, Illinois 60208, United States
# Department of Mechanical Engineering and the Materials Science and Engineering Program, The University of Texas at Austin, Austin, Texas 78712, United States
△ Department of Chemistry and Biochemistry, University of Notre Dame, Notre Dame, Indiana 46556, United States
▼ Department of Materials Science and Engineering, Cornell University, Ithaca, New York 14853, United States
▲ Department of Electrical Engineering and Computer Sciences, University of California, Berkeley, California 94720, United States
▽ Department of Physics, Case Western Reserve University, Cleveland, Ohio 44106, United States
○ Department of Mechanical Engineering, The University of Texas at Austin, Austin, Texas 78712, United States
● Department of Electrical and Computer Engineering, Cornell University, Ithaca, New York 14850, United States
□ Department of Physics, The Pennsylvania State University, University Park, Pennsylvania 16802, United States
■ Department of Materials Science and Engineering, The Ohio State University, Columbus, Ohio 43210, United States
*Address correspondence to [email protected]
Cite this: ACS Nano 2013, 7, 4, 2898–2926
Publication Date (Web):March 6, 2013
https://doi.org/10.1021/nn400280c
Copyright © 2013 American Chemical Society
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    Abstract

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    Graphene’s success has shown that it is possible to create stable, single and few-atom-thick layers of van der Waals materials, and also that these materials can exhibit fascinating and technologically useful properties. Here we review the state-of-the-art of 2D materials beyond graphene. Initially, we will outline the different chemical classes of 2D materials and discuss the various strategies to prepare single-layer, few-layer, and multilayer assembly materials in solution, on substrates, and on the wafer scale. Additionally, we present an experimental guide for identifying and characterizing single-layer-thick materials, as well as outlining emerging techniques that yield both local and global information. We describe the differences that occur in the electronic structure between the bulk and the single layer and discuss various methods of tuning their electronic properties by manipulating the surface. Finally, we highlight the properties and advantages of single-, few-, and many-layer 2D materials in field-effect transistors, spin- and valley-tronics, thermoelectrics, and topological insulators, among many other applications.

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