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Enhancement and Quenching Regimes in Metal−Semiconductor Hybrid Optical Nanosources

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Laboratoire de Nanotechnologie et d’Instrumentation Optique, ICD CNRS FRE 2848, Université de Technologie de Troyes BP 2060 Troyes cedex, France
* Address correspondence to [email protected]
Cite this: ACS Nano 2010, 4, 2, 759–764
Publication Date (Web):January 5, 2010
https://doi.org/10.1021/nn901294d
Copyright © 2010 American Chemical Society

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    Abstract

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    We report on the emission of hybrid nanosources composed of gold nanoparticles coupled with quantum dots. The emission relies on energy transfer from the quantum dots to gold nanoparticles which could be de-excited through radiative plasmon relaxation. The dependence of the emission efficiency is studied systematically as a function of the size of gold nanoparticles and interdistance between gold nanoparticles and quantum dots. We demonstrate a size-dependent transition between quenching and enhancement and a nonradiative energy transfer from the quantum dots to the gold nanoparticles.

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