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Oxygen Concentration Control of Dopamine-Induced High Uniformity Surface Coating Chemistry

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    Oxygen Concentration Control of Dopamine-Induced High Uniformity Surface Coating Chemistry
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    † WCU Department of Energy Engineering, Hanyang University, Seoul 133-791, Republic of Korea
    § IBM Almaden Research Center, San Jose, California 95120, United States
    ∥ LG Electronics, Advanced Research Institute, 16 Woomsyeon-dong, Seocho-gu, Seoul 137-724, Republic of Korea
    ⊥ Department of Chemical Engineering Center for Energy and Environmental Resources, University of Texas at Austin, 10100 Burnet Road, Building 133, Austin, Texas 78758, United States
    *E-mail: [email protected]
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    ACS Applied Materials & Interfaces

    Cite this: ACS Appl. Mater. Interfaces 2013, 5, 2, 233–238
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    https://doi.org/10.1021/am302439g
    Published December 31, 2012
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    Abstract

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    Material surface engineering has attracted great interest in important applications, including electronics, biomedicine, and membranes. More recently, dopamine has been widely exploited in solution-based chemistry to direct facile surface modification. However, unsolved questions remain about the chemical identity of the final products, their deposition kinetics and their binding mechanism. In particular, the dopamine oxidation reaction kinetics is a key to improving surface modification efficiency. Here, we demonstrate that high O2 concentrations in the dopamine solution lead to highly homogeneous, thin layer deposition on any material surfaces via accelerated reaction kinetics, elucidated by Le Chatelier’s principle toward dopamine oxidation steps in a Michael-addition reaction. As a result, highly uniform, ultra-smooth modified surfaces are achieved in much shorter deposition times. This finding provides new insights into the effect of reaction kinetics and molecular geometry on the uniformity of modifications for surface engineering techniques.

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    Cite this: ACS Appl. Mater. Interfaces 2013, 5, 2, 233–238
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