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    Single-Particle Characterization of Summertime Arctic Aerosols Collected at Ny-Ålesund, Svalbard
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    Department of Chemistry, Inha University, YonghyunDong, NamGu, 402-751, Incheon, Korea, Research Center of Environmental Science and Engineering, Shanxi University, Taiyuan, 030006, China, and Department of Mechanical Engineering, Hanyang University, Sangnok-gu, 425-791, Ansan, Korea
    * Corresponding author phone: +82 32 860 7676; fax: +82 32 867 5604; e-mail: [email protected]
    †Inha University.
    ‡Shanxi University.
    §Hanyang University.
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    Environmental Science & Technology

    Cite this: Environ. Sci. Technol. 2010, 44, 7, 2348–2353
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    https://doi.org/10.1021/es903268j
    Published March 3, 2010
    Copyright © 2010 American Chemical Society
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    Abstract

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    Single-particle characterization of summertime Arctic aerosols is useful to understand the impact of air pollutants on the polar atmosphere. In the present study, a quantitative single particle analytical technique, low-Z particle electron probe X-ray microanalysis, was used to characterize 8100 individual particles overall in 16 sets of aerosol samples collected at Ny-Ålesund, Svalbard, Norway on 25−31 July, 2007. Based on their X-ray spectral and secondary electron image data of individual particles, 13 particle types were identified, in which particles of marine origin were the most abundant, followed by carbonaceous and mineral dust particles. A number of aged (reacted) sea salt (and mixture) particles produced by the atmospheric reaction of genuine sea-salts, especially with NOx or HNO3, were significantly encountered in almost all the aerosol samples. They greatly outnumbered genuine sea salt particles, implying that the summertime Arctic atmosphere, generally regarded as a clean background environment, is disturbed by anthropogenic air pollutants. The main sources of airborne NOx (or HNO3) are probably ship emissions around the Arctic Ocean, industry emission from northern Europe and northwestern Siberia, and renoxification of NO3− within or on the melting snow/ice surface.

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    Cite this: Environ. Sci. Technol. 2010, 44, 7, 2348–2353
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    https://doi.org/10.1021/es903268j
    Published March 3, 2010
    Copyright © 2010 American Chemical Society
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