Wrinkled Ultrathin Graphitic C3N4 Nanosheets for Photocatalytic Degradation of Organic WastewaterClick to copy article linkArticle link copied!
- Mingming GaoMingming GaoKey Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR ChinaMore by Mingming Gao
- Jing Feng*Jing Feng*Tel: +86-451-82569890. Fax: +86-451-82533026. E-mail: [email protected]Key Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR ChinaMore by Jing Feng
- Zhiqiang ZhangZhiqiang ZhangKey Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR ChinaMore by Zhiqiang Zhang
- Mengzhen GuMengzhen GuKey Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR ChinaMore by Mengzhen Gu
- Jinxin WangJinxin WangKey Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR ChinaMore by Jinxin Wang
- Wenjing ZengWenjing ZengKey Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR ChinaMore by Wenjing Zeng
- Yanzhuo LvYanzhuo LvKey Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR ChinaMore by Yanzhuo Lv
- Yueming RenYueming RenKey Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR ChinaMore by Yueming Ren
- Tong WeiTong WeiKey Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR ChinaMore by Tong Wei
- Zhuangjun Fan*Zhuangjun Fan*Tel: +86-451-82569890. Fax: +86-451-82533026. E-mail: [email protected]Key Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR ChinaMore by Zhuangjun Fan
Abstract
![Abstract Image](/cms/10.1021/acsanm.8b01528/asset/images/medium/an-2018-01528g_0010.gif)
Wrinkled ultrathin graphitic C3N4 nanosheets (U-g-C3N4) have been successfully synthesized via a thermal condensation process and subsequent rapid cooling treatment in liquid nitrogen. The layer contraction force caused by the rapid cooling process can break the van der Waals forces between the interlayers, thus successfully exfoliating the bulk g-C3N4. The U-g-C3N4 exhibits large specific surface area, effective separation of the photogenerated carriers, and increased visible-light absorbance, which can promote the quantity and lifetime of the photoexcited electrons, resulting in a high photodegradation efficiency of 99.82%. These results show that the interlayer contraction force is a viable option for exfoliating layered materials into a thin-layer structure. This is an interesting and easy method for obtaining thin-layer materials.
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