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Wrinkled Ultrathin Graphitic C3N4 Nanosheets for Photocatalytic Degradation of Organic Wastewater

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Download Hi-Res ImageDownload to MS-PowerPointCite This:ACS Appl. Nano Mater. 2018, 1, 12, 6733-6741
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    Wrinkled Ultrathin Graphitic C3N4 Nanosheets for Photocatalytic Degradation of Organic Wastewater
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    • Mingming Gao
      Mingming Gao
      Key Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR China
      More by Mingming Gao
    • Jing Feng*
      Jing Feng
      Key Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR China
      *Tel: +86-451-82569890. Fax: +86-451-82533026. E-mail: [email protected]
      More by Jing Feng
      Orcidhttp://orcid.org/0000-0001-5997-828X
    • Zhiqiang Zhang
      Zhiqiang Zhang
      Key Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR China
      More by Zhiqiang Zhang
    • Mengzhen Gu
      Mengzhen Gu
      Key Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR China
      More by Mengzhen Gu
    • Jinxin Wang
      Jinxin Wang
      Key Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR China
      More by Jinxin Wang
    • Wenjing Zeng
      Wenjing Zeng
      Key Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR China
      More by Wenjing Zeng
    • Yanzhuo Lv
      Yanzhuo Lv
      Key Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR China
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    • Yueming Ren
      Yueming Ren
      Key Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR China
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    • Tong Wei
      Tong Wei
      Key Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR China
      More by Tong Wei
    • Zhuangjun Fan*
      Zhuangjun Fan
      Key Laboratory of Superlight Materials & Surface Technology of Ministry of Education, Harbin Engineering University, Harbin 150001, PR China
      *Tel: +86-451-82569890. Fax: +86-451-82533026. E-mail: [email protected]
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    ACS Applied Nano Materials

    Cite this: ACS Appl. Nano Mater. 2018, 1, 12, 6733–6741
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    https://doi.org/10.1021/acsanm.8b01528
    Published November 21, 2018
    Copyright © 2018 American Chemical Society
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    Abstract

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    Wrinkled ultrathin graphitic C3N4 nanosheets (U-g-C3N4) have been successfully synthesized via a thermal condensation process and subsequent rapid cooling treatment in liquid nitrogen. The layer contraction force caused by the rapid cooling process can break the van der Waals forces between the interlayers, thus successfully exfoliating the bulk g-C3N4. The U-g-C3N4 exhibits large specific surface area, effective separation of the photogenerated carriers, and increased visible-light absorbance, which can promote the quantity and lifetime of the photoexcited electrons, resulting in a high photodegradation efficiency of 99.82%. These results show that the interlayer contraction force is a viable option for exfoliating layered materials into a thin-layer structure. This is an interesting and easy method for obtaining thin-layer materials.

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    Cited By

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    This article is cited by 75 publications.

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    Cite this: ACS Appl. Nano Mater. 2018, 1, 12, 6733–6741
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